Laser-Liquid Interaction in Laser-Induced Forward Transfer (LIFT) Printing: A Multiscale Perspective on Bubble Dynamics and Material Ejection
激光诱导前向转移打印中的激光-液体相互作用:气泡动力学与材料喷射的多尺度视角
Shuqi Zhou, Abdol Hadi Mokarizadeh, Ben Xu
AI总结 本文从多尺度视角综述激光诱导前向转移打印中气泡动力学与材料喷射的耦合机制,分析供体架构、激光参数、材料流变等对气泡成核、射流形成及沉积的影响,并讨论建模方法。
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激光诱导前向转移(LIFT)是一种无喷嘴的激光辅助打印方法,为功能性墨水、纳米颗粒悬浮液、聚合物、水凝胶、生物材料及其他难以通过喷嘴配制的材料提供了一种先进制造途径。然而,LIFT的表面简单性掩盖了强耦合的激光-液体相互作用。激光能量在受限的供体结构内被吸收,转化为热和等离子体响应,然后转化为供体材料的气泡介导运动。空化气泡提供了光能沉积与流体动力学喷射过程之间的瞬态机械桥梁。本章从气泡动力学和材料喷射的多尺度视角呈现LIFT。首先回顾了主要的LIFT供体架构。然后,考察了供体带设计、吸收层特性、激光参数、材料流变性如何控制气泡成核/生长、射流形成、液滴破碎和最终沉积。讨论了建模方法作为连接跨时间和长度尺度实验观测的工具,范围从降阶估计到界面分辨模拟和数据驱动过程图。作为一个说明性的机理示例,简要比较了纯热、等离子体介导以及耦合等离子体-热-热弹性框架下的早期气泡成核,以展示不同的成核假设如何为下游气泡生长和射流模型提供初始条件。本章最后指出了基于中间气泡和射流可观测量的气泡感知供体设计、时间分辨诊断、基准数据集和预测性LIFT过程图的机会。
Laser-induced forward transfer (LIFT) is a nozzle-free laser-assisted printing method that provides an advanced manufacturing route for spatially selective deposition of functional inks, nanoparticle suspensions, polymers, hydrogels, biological materials, and other difficult-to-nozzle formulations. The apparent simplicity of LIFT, however, conceals a strongly coupled laser-liquid interaction. Laser energy is absorbed within a confined donor architecture, converted into thermal and plasma responses, and then transformed into bubble-mediated motion of the donor material. The cavitation bubble provides the transient mechanical bridge between optical energy deposition and the hydrodynamic ejection process. This chapter presents LIFT from a multiscale perspective centered on bubble dynamics and material ejection. It first reviews major LIFT donor architectures. Then, it examines how donor ribbon design, absorbing-layer properties, laser parameters, material rheology, control bubble inception/growth, jet formation, droplet breakup, and final deposition. Modeling approaches are discussed as tools for connecting experimental observations across time and length scales, ranging from reduced-order estimates to interface-resolving simulations and data-driven process maps. As one illustrative mechanistic example, thermal-only, plasma-mediated, and coupled plasma-thermal-thermoelastic frameworks for early-stage bubble inception are briefly compared to show how different inception assumptions can provide initial conditions for downstream bubble growth and jetting models. This chapter concludes by identifying opportunities for bubble-aware donor design, time-resolved diagnostics, benchmark datasets, and predictive LIFT process maps based on intermediate bubble and jet observables.