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2606.12527 2026-06-12 quant-ph cond-mat.stat-mech cond-mat.str-el 新提交

Statistical Mechanics and Symmetries of Non-Abelian Anyon Proliferation: From Deformation to Decoherence

非阿贝尔任意子增殖的统计力学与对称性:从形变到退相干

Avi Vadali, Robijn Vanhove, Ruben Verresen, Jason Alicea, Pablo Sala

AI总结 通过统计力学模型和蒙特卡洛模拟,研究非阿贝尔任意子增殖导致拓扑序失稳的机制,发现两个非阿贝尔任意子物种的增殖会寄生凝聚共享的阿贝尔融合结果,破坏拓扑序。

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AI中文摘要

拓扑量子计算依赖于编织非阿贝尔任意子,但要求底层拓扑序在非完美态制备和环境噪声下存活。我们证明,拓扑序对波函数形变和退相干(后者通过综合征分布探测)的不稳定性通常由统计力学模型描述,其对称性自然揭示出破坏性的任意子激发。例如,我们将此框架与蒙特卡洛模拟结合,解决了$D_4$拓扑序在形变和量子通道(增殖多个单独无法凝聚的非阿贝尔任意子物种)下的稳定性问题。我们证明,超过有限阈值后,两个非阿贝尔任意子物种的增殖会寄生凝聚一个共享的阿贝尔任意子融合结果,从而破坏拓扑序。我们的基于对称性的方法将由此产生的平凡相与凝聚所有阿贝尔电荷得到的平凡相明确区分;换言之,平凡相“记住”了哪些任意子凝聚。该框架为基于综合征测量识别非阿贝尔拓扑序最优解码器的相关对称性迈出了第一步。

英文摘要

Topological quantum computation relies on braiding non-Abelian anyons, but requires the underlying topological order to survive imperfect state preparation and environmental noise. We show that the instability of topological order to wavefunction deformations and to decoherence, with the latter probed by syndrome distributions, are generically captured by stat-mech models whose symmetries naturally expose the corrupting anyonic excitations. As an example, we combine this framework with Monte-Carlo simulations to resolve the stability of $D_4$ topological order under deformations and quantum channels that proliferate multiple non-Abelian anyon species that individually are unable to condense. We show that beyond a finite threshold, proliferation of two non-Abelian anyon species parasitically condenses a shared Abelian-anyon fusion outcome, destroying the topological order. Our symmetry-based approach sharply differentiates the resulting trivial phase from that obtained by condensing all Abelian charges; in other words, the trivial phase "remembers" which anyons condensed. This framework provides a first step into identifying the relevant symmetry for optimal decoders, conditioned on syndrome measurements, of non-Abelian topological order.

2606.12526 2026-06-12 hep-th cond-mat.stat-mech quant-ph 新提交

Multi-entropy in heavy local quenches

重局域淬火中的多重熵

Kosei Fujiki, Kenya Tasuki

AI总结 研究二维全息共形场论中重局域淬火后三体纠缠的时间演化,通过微扰和全反作用几何分析发现,真正多重熵由全局鞍点选择而非局域能量响应控制。

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38 pages, 9 figures
AI中文摘要

我们研究了二维全息共形场论中重局域淬火后三体纠缠的时间演化。我们的诊断是相邻区间的真正多重熵,从体和边界两个角度计算。微扰体分析表明,真空测地线网络周围的一阶小质量扰动在淬火后的任何时间都相同抵消。在完全反作用的几何中,真空减除的真正多重熵源于三叉测地线网络选择的缠绕与成对测地线独立选择的缠绕之间的不匹配。在尖锐淬火极限下,真正多重熵的时间依赖性运动学上固定为时间有理函数的对数,并且与重算子维度无关。CFT计算在重-光真空块近似内重现了相同的公式,其中重背景均匀化映射中的分支选择对应于体中的缠绕选择。这些结果表明,在此设置中,真正多重熵由全局鞍点选择控制,而不是由局域能量响应或准粒子传播控制。

英文摘要

We study the time evolution of tripartite entanglement in heavy local quenches in two-dimensional holographic conformal field theories. Our diagnostic is the genuine multi-entropy of adjacent intervals, computed from both bulk and boundary perspectives. A perturbative bulk analysis shows that the first-order small-mass perturbation around the vacuum geodesic network cancels identically at any time after the quench. In the fully back-reacted geometry, a vacuum-subtracted genuine multi-entropy arises from a mismatch between the winding selected by the trivalent geodesic network and the windings selected independently by the pairwise geodesics. In the sharp quench limit, the time dependence of genuine multi-entropy is kinematically fixed to logarithms of rational functions of time and is independent of the heavy operator dimension. The CFT calculation reproduces the same formula within the heavy-light vacuum block approximation, where the branch choice in the heavy-background uniformization map corresponds to the winding selection in the bulk. These results indicate that, in this setup, the genuine multi-entropy is controlled by global saddle selection, rather than by a local energy response or quasiparticle propagation.

2606.12510 2026-06-12 hep-th cond-mat.str-el hep-lat 新提交

Infinite-Order Lattice Chiral Anomalies and CPT

无穷阶格点手征反常与CPT

Elijah Lew-Smith, Salvatore D. Pace, Shu-Heng Shao

AI总结 本文研究格点手征对称性的反常阶数,发现CPT对称性将Onsager反常从二阶提升至无穷阶,更忠实于连续手征反常,并讨论了相应的对称保护拓扑相。

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Comments
17 pages
AI中文摘要

全局对称性反常的一个关键性质是其阶数:使$n$拷贝系统的对角对称性无反常的最小整数$n$。虽然许多常见的格点反常具有有限阶,但连续理论中的微扰反常——由费曼图捕获的那些——具有无穷阶。在本文中,我们展示了Onsager对称性,即1+1d无质量狄拉克费米子的手征对称性的格点实现,具有二阶反常。然而,施加格点CPT对称性将此反常从二阶提升至无穷阶,产生一个更忠实地匹配连续手征反常的格点手征对称性结构。我们还讨论了这些无穷阶格点反常对应的2+1d对称保护拓扑相。

英文摘要

A key property of a global symmetry's anomaly is its order: the smallest integer $n$ for which the diagonal symmetry of the $n$-copy system is anomaly-free. While many familiar lattice anomalies have finite order, perturbative anomalies in the continuum$-$those captured by Feynman diagrams$-$have infinite order. In this paper, we show that the Onsager symmetry, a lattice realization of the chiral symmetry of a 1+1d massless Dirac fermion, has an order-two anomaly. However, imposing lattice CPT symmetry enhances this anomaly from order two to infinite order, yielding a lattice chiral symmetry structure that more faithfully matches the continuum chiral anomaly. We also discuss the corresponding 2+1d symmetry-protected topological phases for these infinite-order lattice anomalies.

2606.12478 2026-06-12 cs.LG cond-mat.stat-mech quant-ph 新提交

Boltzmann Attention: Learnable Ising Couplings for Cooperative Attention

玻尔兹曼注意力:用于协同注意力的可学习伊辛耦合

Gilhan Kim, Daniel K. Park

发表机构 * Yonsei University(延世大学)

AI总结 提出玻尔兹曼注意力,通过可学习的伊辛耦合增强注意力机制中的位置间交互,在字符级语言建模和括号匹配任务中优于标准softmax注意力,并展示了量子退火训练的有效性。

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19 pages, 5 figures
AI中文摘要

注意力机制是现代序列模型的核心,但标准注意力主要通过单个查询-键相似度计算相关性。尽管softmax归一化引入了位置间的竞争,但标准注意力层并未显式参数化注意力决策之间的可学习交互。这限制了其直接在注意力机制内建模协同或对抗性共注意力结构的能力。我们提出玻尔兹曼注意力,一种基于能量的泛化,其中注意力模式由相互作用的伊辛模型控制。该方法用可学习的成对耦合增强通常的数据依赖局部场,使模型能够表示超出softmax或sigmoid注意力所捕获的位置间相关性。在字符级语言建模和合成括号匹配实验上,玻尔兹曼注意力在标准Transformer架构中持续优于标准softmax注意力,且优势随序列长度增加而更加明显。四路消融实验证实改进来自可学习的成对耦合。这些结果表明,显式位置间交互为基于注意力的序列建模提供了原则性增强。此外,伊辛公式为基于量子计算的采样策略开辟了自然路径:我们证明非绝热量子退火提供了实用的训练方法,同时保持了与精确玻尔兹曼计算相当的性能。

英文摘要

Attention mechanisms are central to modern sequence models, yet standard attention computes relevance primarily through individual query--key similarities. Although softmax normalization introduces competition among positions, a standard attention layer does not explicitly parameterize learnable interactions between attention decisions. This limits its ability to directly model cooperative or antagonistic co-attention structure within the attention mechanism itself. We propose Boltzmann attention, an energy-based generalization in which attention patterns are governed by an interacting Ising model. The method augments the usual data-dependent local fields with learnable pairwise couplings, allowing the model to represent inter-position correlations beyond those captured by softmax or sigmoid attention. Experiments on character-level language modeling and synthetic bracket matching show that Boltzmann attention consistently improves over standard softmax attention within a standard Transformer architecture, with the advantage becoming more pronounced as sequence length increases. A four-way ablation confirms that the improvement arises from the learnable pairwise couplings. These results suggest that explicit inter-position interactions provide a principled enhancement for attention-based sequence modeling. Moreover, the Ising formulation opens a natural path toward quantum-computing-based sampling strategies: we demonstrate that diabatic quantum annealing provides a practical training method while maintaining competitive performance with exact Boltzmann computation.

2606.13664 2026-06-12 cond-mat.mtrl-sci 新提交

Morphology control and low-temperature magnetotransport in chiral 2D perovskite R-(MBA)$_2$PbI$_4$

手性二维钙钛矿R-(MBA)$_2$PbI$_4$的形貌控制与低温磁输运

Shehreen Aslam, Sam Saiter, Bradley Lloyd, Paul Kliewer, Matthew P. Hautzinger, Matthew C. Beard, Meenakshi Singh

AI总结 通过工程化手性钙钛矿薄膜形貌,首次实现横向器件集成,在霍尔棒结构中测量到空穴迁移率约0.2 cm²/V·s和载流子密度约3×10¹⁴ cm⁻²,并观察到晶界增强磁阻效应。

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20 pages, 4 figures, supplemental information
AI中文摘要

二维手性杂化钙钛矿,如R/S-(MBA)\textsubscript{2}PbI\textsubscript{4},是研究和实现手性依赖电荷与自旋输运的领先候选材料。然而,其过大的面内电阻阻碍了电学表征。这里,我们通过工程化手性钙钛矿$R\text{-(MBA)}_2\text{PbI}_4$的薄膜形貌克服了这一瓶颈,实现了首次稳健的横向器件集成。在霍尔棒结构中,我们在暗条件下进行了霍尔测量,明确识别出p型导电,霍尔迁移率约为$0.2 \text{cm}^2 \text{V}^{-1} \text{s}^{-1}$,载流子密度约为$3\times10^{14} \text{ cm}^{-2}$,这些参数在此类材料中此前无法获得。此外,我们观察到沿穿过晶界的输运路径磁阻增强,突显了形貌对面内输运的强烈影响。本工作展示了面内磁输运,为未来研究手性诱导自旋选择性(CISS)的基本机制以及加速手性材料集成到功能性自旋电子器件中铺平了道路。

英文摘要

Two-dimensional chiral hybrid perovskites, such as R/S-(MBA)\textsubscript{2}PbI\textsubscript{4}, are leading candidates for realizing and studying chirality-dependent charge and spin transport. However, their prohibitive in-plane resistance has precluded the electrical characterization. Here, we overcome this bottleneck by engineering the thin-film morphology of the chiral perovskite $R\text{-(MBA)}_2\text{PbI}_4$, enabling the first robust lateral device integration. In Hall-bar geometries, we demonstrate Hall measurements under dark conditions, unambiguously identifying p-type conduction with a Hall mobility of $\sim 0.2 \text{cm}^2 \text{V}^{-1} \text{s}^{-1}$ and a carrier density of $\sim 3\times10^{14} \text{ cm}^{-2}$, parameters previously inaccessible in this class of materials. Furthermore, we observe enhanced magnetoresistance along transport paths crossing grain boundaries, highlighting the strong influence of morphology on in-plane transport. This work demonstrates in-plane magnetotransport, enabling future investigations of the fundamental mechanisms of chirality-induced spin selectivity (CISS) and accelerating the integration of chiral materials into functional spintronic devices.

2606.13651 2026-06-12 cond-mat.mes-hall cond-mat.str-el 新提交

Engineering electrically-switchable quantum anomalous Hall states by spin-orbit coupling

通过自旋-轨道耦合工程实现电可切换的量子反常霍尔态

Maosen Qin, Ziwei Wang, Gyeongmin Kim, Kenji Watanabe, Takashi Taniguchi, Steven H. Simon, Siddharth A. Parameswaran, Hryhoriy Polshyn

AI总结 通过WSe2邻近耦合诱导自旋-轨道耦合,调控扭转单层-双层石墨烯的磁化反转,实现量子反常霍尔态的非易失性电切换,并展示Chern数在|C|=2和1之间的栅极可调性。

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22 pages, 15 figures
AI中文摘要

石墨烯莫尔系统中非易失性栅极驱动的量子反常霍尔(QAH)态切换为基于手征边缘态的拓扑电子学提供了有前景的途径。然而,有意利用这种切换机制需要控制QAH态的磁性和亚稳性。虽然先前的演示主要依赖于莫尔器件的内在磁能景观,但这里我们表明,这种景观可以通过与WSe2的邻近耦合来工程化。我们发现,通过WSe2邻近化扭转单层-双层石墨烯重塑了负责QAH态非易失性电切换的磁化反转。我们将此效应归因于邻近诱导的自旋-轨道耦合(SOC),它可以锁定自旋和谷,并改变与切换相关的竞争态的磁化,相比于非邻近化的石墨烯系统。我们的发现确立了邻近诱导的SOC作为一种在石墨烯基系统中工程化磁性和可切换磁态的新方法。我们进一步证明,tMBG中的强磁亚稳性允许磁态在QAH和金属态之间,以及在Chern数|C|=2和1的QAH态之间进行栅极调谐,而无需重置磁态。这一功能指向了基于QAH手征边缘态的新型器件架构。

英文摘要

Nonvolatile gate-driven switching of quantum anomalous Hall (QAH) states in graphene moiré systems provides a promising route toward topological electronics based on chiral edge states. However, deliberate use of this switching mechanism requires control over both the magnetic properties and metastability of QAH states. While previous demonstrations mostly relied on the intrinsic magnetic energy landscape of moiré devices, here we show that this landscape can be engineered through proximity coupling to WSe2. We find that proximitizing twisted monolayer-bilayer graphene by WSe2 reshapes the magnetization reversals responsible for nonvolatile electrical switching of QAH states. We attribute this effect to the proximity-induced spin-orbit coupling (SOC), which can lock spin and valley and modify the magnetization of the competing states involved in switching compared with non-proximitized graphene systems. Our findings establish proximity-induced SOC as a new way to engineer magnetic properties and switchable magnetic states in graphene-based systems. We further demonstrate that strong magnetic metastability in tMBG allows the magnetic states to be gate-tuned between QAH and metallic regimes, and between QAH states with Chern numbers |C| = 2 and 1 without resetting the magnetic state. This functionality points toward new device architectures based on QAH chiral edge states.

2606.13645 2026-06-12 cond-mat.quant-gas 新提交

Driven dynamics of an attractive Bose polaron

吸引性玻色极化子的驱动动力学

Saptarshi Majumdar, Aleksandra Petković

AI总结 研究一维均匀弱相互作用玻色子系统中杂质在恒外力下的非平衡动力学,发现杂质在无晶格时呈现漂移布洛赫振荡,并分析漂移速度、振幅等随力的变化规律。

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11 pages, 11 figures
AI中文摘要

我们研究了一维空间中均匀弱相互作用玻色子系统中,受恒定外力驱动的杂质的非平衡动力学。假设杂质-玻色子相互作用是吸引性的。我们证明,在没有晶格的情况下,杂质在广泛的力范围内表现出漂移布洛赫振荡。我们表征了宿主玻色子的动力学响应,并解释了布洛赫振荡的机制。我们分析了在广泛的力和其他系统参数下漂移速度、布洛赫振幅和振荡周期的行为。与排斥性杂质-玻色子相互作用的情况相反,漂移速度对弱施加力呈现亚线性依赖,$V_d\sim {F}^{\alpha}$,其中指数$\alpha$为正且小于1。漂移速度随力单调增加,尽管在不同$F$区域缩放行为变化显著。此外,速度振荡的振幅表现出丰富的行为:它首先随力衰减,达到最小值,然后复苏,随力增加。

英文摘要

We study the out-of-equilibrium dynamics of an impurity driven by a constant external force through a system of homogeneous weakly-interacting bosons in one spatial dimension. The impurity-boson interaction is assumed to be attractive. We show that the impurity exhibits drifted Bloch oscillations in a wide range of forces in the absence of a lattice. We characterize the dynamical response of the host bosons and explain the mechanism underlying the Bloch oscillations. We analyse the behavior of the drift velocity, the Bloch amplitude and the time period of oscillations in a wide range of forces and other system parameters. In contrast to the case of repulsive impurity-boson interaction, the drift velocity exhibits a sub-linear dependence on a weak applied force, $V_d\sim {F}^{\alpha}$ with a positive exponent $\alpha$ smaller than unity. The drift velocity monotonically increases with force, though the scaling behavior varies considerably across different regimes of $F$. Moreover, the amplitude of the velocity oscillations displays rich behavior: it first undergoes a decay with force, reaches a minimum, and then presents a revival, increasing with force.

2606.13617 2026-06-12 cond-mat.soft cond-mat.stat-mech 新提交

Geometric formulation of state-dependent Langevin dynamics using scalar free energy

使用标量自由能的状态依赖朗之万动力学的几何表述

Kento Yasuda, Zhongqiang Xiong, Zhanglin Hou, Kenta Ishimoto, Xinpeng Xu, Shigeyuki Komura

AI总结 本文通过引入标量自由能并将扩散张量作为构型空间的度量,提出了几何一致的朗之万方程,明确了坐标协变性,并展示了在坐标变换、几何约束和投影等例子中的一致性。

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AI中文摘要

具有状态依赖扩散的随机动力学广泛应用于受限、各向异性和流体动力学耦合系统中的布朗运动。传统的朗之万表述包含与乘性噪声相关的虚假漂移,但其自由能通常不按标量变换,这意味着协变性不明确。这里,我们通过引入标量自由能并使用扩散张量作为构型空间的度量,公式化了几何一致的朗之万方程。虚假漂移随后被表示为扩散度量的克里斯托费尔贡献。虽然我们的表述通过非标量和标量自由能之间的关系等价于传统表述,但它明确了坐标协变性。我们在状态依赖扩散的代表性例子中展示了其一致性,这些例子源于坐标变换、几何约束以及从弯曲空间到平坦空间的投影。

英文摘要

Stochastic dynamics with state-dependent diffusion are widely used for Brownian motion in confined, anisotropic, and hydrodynamically coupled systems. The conventional Langevin formulation includes a spurious drift associated with multiplicative noise, but its free energy generally does not transform as a scalar, meaning that the covariance is not explicit. Here, we formulate a geometrically consistent Langevin equation by introducing a scalar free energy and using the diffusion tensor as a metric on configuration space. The spurious drift is then expressed as a Christoffel contribution of the diffusion metric. While our formulation is equivalent to the conventional one through the relation between the non-scalar and scalar free energies, it makes the coordinate covariance explicit. We demonstrate its consistency in representative examples of state-dependent diffusion arising from coordinate transformations, geometrical confinement, and projection from curved to flat spaces.

2606.13588 2026-06-12 cond-mat.mtrl-sci 新提交

Cepstral Analysis to accelerate Green-Kubo thermal conductivity calculations of Metal-Organic Frameworks

倒谱分析加速金属有机框架的Green-Kubo热导率计算

Florian P. Lindner (1), Egbert Zojer (1), Sandro Wieser (2) ((1) Institute of Solid State Physics, Graz University of Technology (2) Institute of Materials Chemistry, TU Wien)

AI总结 针对金属有机框架热导率计算中统计噪声大、参数依赖性强的问题,提出倒谱分析与Green-Kubo模拟结合的方法,在缩短采样时间的同时获得稳定结果。

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AI中文摘要

金属有机框架(MOFs)是有前景的多孔材料,用于气体存储和分离等应用,其中热传输会严重影响器件性能。然而,其热导率的可靠计算预测仍然具有挑战性。特别是,基于平衡分子动力学的Green-Kubo(GK)模拟作为最广泛使用的方法,受到统计噪声的严重影响。此外,它们依赖于多个模糊的用户定义参数,这阻碍了可转移性和自动化。在这里,我们针对金属有机框架证明,倒谱分析与GK模拟相结合提供了一条稳健的途径,可以大规模缓解这些问题,同时减少所需的采样时间。这在三种原型框架MOF-5、HKUST-1和ZIF-8上得到了展示,使用了基于DFT参考数据训练的机器学习矩张量势。与传统的直接GK分析相比,后者表现出不稳定的收敛性和对临时参数选择的强烈敏感性,倒谱方法在广泛的相关长度范围内产生稳定的结果,并在约1-2纳秒的总采样时间内实现收敛。这确立了基于倒谱分析的Green-Kubo模拟与机器学习势相结合,作为用于MOFs和其他复杂低热导率材料中热传输的近从头算精度预测的高效、可重复且自动化就绪的框架。

英文摘要

Metal-organic frameworks (MOFs) are promising porous materials for applications such as gas storage and separation, where heat transport can critically affect device performance. However, reliable computational prediction of their thermal conductivities remains challenging. In particular, equilibrium molecular-dynamics-based Green-Kubo (GK) simulations, as the most widely used approach, are severely affected by statistical noise. Moreover, they rely on multiple ambiguous, user-defined parameters, which hinder transferability and automation. Here, we demonstrate for metal-organic frameworks that cepstral analysis in combination with GK simulations provides a robust route to massively mitigate these problems, while simultaneously reducing the required sampling times. This is shown for three prototypical frameworks, MOF-5, HKUST-1, and ZIF-8, employing machine-learned moment tensor potentials trained on DFT reference data. In contrast to conventional, direct GK analysis, which shows erratic convergence and strong sensitivity to ad hoc choices of parameters, the cepstral approach yields stable results across a wide range of correlation lengths and achieves convergence within about 1-2 ns of total sampling time. This establishes cepstral analysis base Green-Kubo simulations combined with machine-learned potentials as an efficient, reproducible and automation-ready framework for near ab initio accuracy prediction of thermal transport in MOFs and other complex low-thermal-conductivity materials.

2606.13586 2026-06-12 cond-mat.soft cond-mat.stat-mech physics.chem-ph 新提交

Exploratory digital alchemy for colloidal crystal discovery

探索性数字炼金术用于胶体晶体发现

Shih-Kuang (Alex)Lee, Sun-Ting Tsai, Sharon C. Glotzer

AI总结 提出探索性数字炼金术(EDA),融合数字炼金术与元动力学,通过释放目标晶体约束并引入探索偏差,自动发现稳定新胶体晶体的势参数。

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Comments
12 pages, 5 figures
AI中文摘要

数字炼金术(DA)由Van Anders等人提出,是一种基于统计力学的广义热力学系综方法,利用计算机模拟优化胶体粒子设计。该方法应用统计力学原理预测和定制粒子属性,以实现所需的自组装结构或材料性质。然而,作为一种逆向设计方法,其主要局限性在于目标结构必须事先已知。因此,DA的最优设计并不能保证目标结构是最稳定或唯一稳定的。这凸显了采用探索性方案进行正向设计以优化新型胶体设计的重要性,在这种情况下更为合适。本文中,我们引入探索性数字炼金术(EDA),一种增强的正向设计方案,首先释放DA中目标晶体的约束,然后引入一种探索导向的偏置,该偏置已广泛用于增强采样方法如元动力学(MetaD)中。我们通过涉及二维Lennard-Jones Gauss势(LJGP)和三维振荡对势(OPP)相互作用的粒子示例展示了EDA的实用性。我们应用EDA研究了不同温度下LJGP不同势参数的自由能景观。通过探索性方案,我们还成功识别了稳定亚稳态Frank-Kasper相的一系列OPP势参数。我们的方法融合了标准DA框架与元动力学,可能对研究广义系综中的炼金术反应有用。

英文摘要

Digital Alchemy (DA), introduced by Van Anders et al., is a statistical mechanics-based generalized thermodynamic ensemble method that employs computer simulations to optimize colloidal particle design. This approach applies the principles of statistical mechanics to predict and tailor particle attributes that lead to desired self-assembled structures or material properties. However, as an inverse design method, its main limitation is that the target structure must be known \textit{a priori}. Therefore, the optimal design from DA does not guarantee the targeted structure is the most or the only stable one. This highlights the importance of forward design with an exploratory scheme for optimizing novel colloid designs, which becomes more suitable in such cases. In this paper, we introduce Exploratory Digital Alchemy (EDA), an enhanced forward design scheme that begins by releasing the constraint of the target crystal from DA, followed by an exploration-oriented bias that has been extensively used in enhanced sampling methods such as metadynamics (MetaD). We demonstrate the utility of EDA through examples involving particles interacting via a two-dimensional Lennard-Jones Gauss potential (LJGP) and a three-dimensional oscillating pair potential (OPP). We applied EDA to study the free energy landscapes given different potential parameters of LJGP at different temperatures. With the exploratory scheme, we've also successfully identified a wide range of OPP potential parameters that stabilize metastable Frank-Kasper phases. Our approach fuses the standard DA framework with metadynamics, which could potentially be useful for studying alchemical reactions in a generalized ensemble.

2606.13584 2026-06-12 cond-mat.soft physics.flu-dyn 新提交

Limits of constant-parameter constitutive models for hydrogels under inertial cavitation

惯性空化下水凝胶常参数本构模型的局限性

Tianyi Chu, Joseph Beckett, Zhiren Zhu, Jonathan B. Estrada, Spencer H. Bryngelson

AI总结 通过改进的迭代集合卡尔曼平滑器,在neo-Hookean Kelvin-Voigt模型框架下,发现水凝胶在空化过程中剪切模量和粘度随时间变化,表明常参数模型不足以描述完整空化事件。

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AI中文摘要

软材料在高应变率下的力学表征因其高柔顺性、非线性粘弹性行为以及潜在的历史依赖响应而具有挑战性。惯性微空化流变学(IMR)通过将激光诱导空化(LIC)实验与气泡动力学模型的数值模拟相结合来推断本构模型和材料参数,从而解决了这一挑战。IMR及其变体推断的参数依赖于所选拟合窗口,这表明常参数本构模型不足以描述完整的空化事件。我们利用这种窗口依赖性来识别常参数假设何时失效,而不是报告单一的有效参数集。使用改进的迭代集合卡尔曼平滑器与多重数据同化(MIEnKS-MDA)在移动、重叠窗口上估计本构参数。在neo-Hookean Kelvin-Voigt(NHKV)本构模型内,我们获得了不同交联剂浓度的聚丙烯酰胺(PAAm)水凝胶中本构响应的时间分辨估计。推断的剪切模量和粘度在空化过程中通常先下降然后趋于平稳,同时表现出相对较弱的温度敏感性。相比之下,对于明胶凝胶,推断的性质演变显示出明显的温度依赖性,在低温和高温下呈现不同趋势。此外,表观剪切模量和粘度在前两次气泡塌陷期间均表现出显著变化。这些结果表明,在指定的NHKV本构结构内进行时间分辨参数估计可以诊断常参数模型假设在空化过程中的不足,从而指导开发改进的基于物理的复杂气泡-材料相互作用模型。

英文摘要

Mechanical characterization of soft materials at high strain rates is challenging due to their high compliance, nonlinear viscoelastic behavior, and potentially history-dependent responses. Inertial microcavitation rheometry (IMR) addresses this challenge by coupling laser-induced cavitation (LIC) experiments with numerical simulations of bubble dynamics models to infer constitutive models and material parameters. Both IMR and its variants infer parameters that depend on the chosen fitting window, which suggests that a constant-parameter constitutive model is insufficient to describe the full cavitation event. We use this window dependence to identify when the constant-parameter assumption fails, rather than to report a single effective parameter set. The constitutive parameters are estimated over moving, overlapping windows using a modified iterative ensemble Kalman smoother with multiple data assimilation (MIEnKS-MDA). Within the neo-Hookean Kelvin--Voigt (NHKV) constitutive model, we obtain time-resolved estimates of the constitutive response in polyacrylamide (PAAm) hydrogels with different crosslinker concentrations. The inferred shear modulus and viscosity generally decrease and then plateau during cavitation, while exhibiting relatively weak temperature sensitivity. For gelatin gels, by contrast, the inferred property evolution shows a pronounced temperature dependence, with distinct trends at low and high temperatures. Moreover, both the apparent shear modulus and viscosity exhibit significant variations during the first two bubble collapses. These results show that time-resolved parameter estimation within the prescribed NHKV constitutive structure can diagnose where the constant-parameter model assumption falls short during cavitation, thereby guiding the development of improved physics-based models of complex bubble--material interactions.

2606.13573 2026-06-12 cond-mat.mtrl-sci 新提交

Tuning perpendicular magnetic anisotropy in ultra-low damping Li$_{0.5}$Al$_{x}$Fe$_{(2.5-x)}$O$_4$ thin films for efficient spin-orbit torque switching

调控超低阻尼Li$_{0.5}$Al$_{x}$Fe$_{(2.5-x)}$O$_4$薄膜的垂直磁各向异性以实现高效自旋轨道矩翻转

Daisy O'Mahoney, Sauviz P. Alaei, Anna Janni, Muzhda Mehrzad, Christoph Klewe, Alpha T. N'Diaye, Zbigniew Galazka, Yuri Suzuki

AI总结 通过外延应变和化学组分调控铁磁尖晶石Li$_{0.5}$Al$_{x}$Fe$_{(2.5-x)}$O$_4$薄膜的垂直磁各向异性,实现超低阻尼(低至$2\ imes10^{-4}$)和低自旋轨道矩翻转电流密度,最佳组分x=0.7为自旋波器件提供平台。

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Comments
8 pages, 6 figures
AI中文摘要

同时具有超低磁振子阻尼、垂直磁各向异性(PMA)和低自旋轨道矩(SOT)翻转电流密度的超薄磁性绝缘体薄膜,对于利用自旋波传输信息而不产生耗散电荷电流的下一代自旋电子学技术是非常理想的,尽管具有挑战性。在这里,我们在铁磁尖晶石Li$_{0.5}$Al$_{x}$Fe$_{(2.5-x)}$O$_4$(LAFO)薄膜中展示了这些性质的组合。通过这个模型系统,我们发现PMA可以通过外延应变以化学组成和衬底选择的形式进行调控,并且低SOT翻转电流密度与较小但有限的PMA相关。超低阻尼主要通过仅具有Fe$^{3+}$作为磁性活性阳离子来稳定,其次是由于Al替代分布引起的无序增加。SOT效率由界面质量决定,与化学组成无关。通过改变Al浓度,我们系统地调控了饱和磁化强度和磁各向异性,同时保持了低至$2\ imes10^{-4}$的超低吉尔伯特阻尼参数和与组成无关的类阻尼SOT效率。我们确定了最佳组成LAFO x=0.7(Li$_{0.5}$Al$_{0.7}$Fe$_{1.8}$O$_4$),它结合了超低阻尼、具有小各向异性场的稳定PMA以及用于SOT翻转的低临界电流密度,使其成为节能自旋波和自旋电子学器件的有前景的材料平台。

英文摘要

Ultra-thin magnetic insulator films that simultaneously exhibit ultra-low magnon damping, perpendicular magnetic anisotropy (PMA), and low spin-orbit torque (SOT) switching current densities are highly desirable, albeit challenging, for next-generation spintronic technologies that exploit spin waves to transport information without dissipative charge currents. Here, we demonstrate this combination of properties in ferrimagnetic spinel Li$_{0.5}$Al$_{x}$Fe$_{(2.5-x)}$O$_4$ (LAFO) thin films. Through this model system, we find that PMA can be tuned by epitaxial strain in the form of chemical composition and substrate choice and that low SOT switching current densities correlate with small but finite PMA. Ultra-low damping is stabilized primarily by having only Fe$^{3+}$ as magnetically active cations with secondary effects due to increased disorder from Al substitution distribution. SOT efficiency is governed by interface quality and independent of chemical composition. By varying the Al concentration, we systematically tune the saturation magnetization and magnetic anisotropy while maintaining ultra-low Gilbert damping parameters as low as $2\times10^{-4}$ and composition-independent damping-like SOT efficiencies. We identify an optimal composition LAFO x=0.7 (Li$_{0.5}$Al$_{0.7}$Fe$_{1.8}$O$_4$), which combines ultra-low damping, stable PMA with small anisotropy fields, and low critical current densities for SOT switching, establishing it as a promising material platform for energy-efficient spin-wave and spintronic devices.

2606.13561 2026-06-12 cond-mat.mtrl-sci 新提交

Lone-Pair-Induced Lattice Softness Enables Ultralow Thermal Conductivity in Hybrid Organic-Inorganic Perovskite GuaPbI$_3$

孤对电子诱导的晶格软化使杂化有机-无机钙钛矿 GuaPbI$_3$ 具有超低热导率

Rudra P. Singh, Shantanu Pathak, Saswata Bhattacharya, R Lakshmi Narayan

AI总结 本文提出基于孤对电子的材料设计策略,通过化学诱导晶格软化在杂化有机-无机钙钛矿 GuaPbI3 中实现超低热导率(0.088 W m^-1 K^-1),同时保持电子传输路径,为热电材料设计提供新原理。

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AI中文摘要

热电冷却效率从根本上受限于晶格热导率,尽管进行了广泛的纳米结构工程,传统无机热电材料已接近性能平台。有机热电材料具有本征低热导率,但通常面临有限且对形态敏感的电荷传输。本文提出一种基于孤对电子的材料设计策略,利用杂化有机-无机钙钛矿中化学诱导的晶格软化。基于物理引导的符号回归机器学习框架识别出与抑制晶格热导率相关的孤对电子主导组分区间,并选择 GuaPbI3 作为候选材料。机械化学合成得到结晶 GuaPbI3,其室温热导率超低,为 kappa = 0.088 W m^-1 K^-1。电学测量揭示了尽管声子被强烈抑制,但仍存在电子活性、偏压依赖的体传导路径,而阻抗谱证实了体主导的传输。密度泛函理论计算表明价带弱色散、价导带不对称性以及晶格内电荷再分布导致的局域静电微环境。计算得到的输运系数表明载流子传输对化学势高度敏感,而洛伦兹数分析表明在带边附近偏离常规的 Wiedemann-Franz 行为。这些结果支持以下图像:富孤对电子的杂化框架产生软且电子异质的晶格环境,抑制声子传输同时保留电子可及态。本工作确立了化学诱导晶格软化作为超低热导率杂化材料的设计原理。

英文摘要

Thermoelectric cooling efficiency is fundamentally constrained by lattice thermal conductivity, yet conventional inorganic thermoelectrics have approached a performance plateau despite extensive nanostructural engineering. Organic thermoelectrics possess intrinsically low thermal conductivity but often suffer from limited and morphology-sensitive charge transport. Here, we introduce a lone-pair-driven materials design strategy based on chemically induced lattice softness in hybrid organic-inorganic perovskites. A physics-guided symbolic-regression-based machine-learning framework identifies a lone-pair-dominated compositional regime associated with suppressed lattice thermal conductivity and selects GuaPbI3 as a candidate material. Mechanochemical synthesis yields crystalline GuaPbI3 with an ultralow room-temperature thermal conductivity of kappa = 0.088 W m^-1 K^-1. Electrical measurements reveal electronically active, bias-dependent bulk conduction pathways despite strong phonon suppression, while impedance spectroscopy confirms bulk-dominated transport. Density functional theory calculations indicate weakly dispersive valence bands, valence-conduction asymmetry, and localized electrostatic microenvironments from charge redistribution within the lattice. Calculated transport coefficients suggest strong sensitivity of carrier transport to chemical potential, while Lorenz-number analysis indicates deviations from conventional Wiedemann-Franz behavior near the band edges. These results support a picture in which lone-pair-rich hybrid frameworks generate soft and electronically heterogeneous lattice environments that suppress phonon transport while preserving electronically accessible states. This work establishes chemically induced lattice softness as a design principle for ultralow-thermal-conductivity hybrid materials.

2606.13548 2026-06-12 cond-mat.mtrl-sci physics.data-an stat.ML 新提交

Symmetry-electronic fingerprints reveal competing magnetic phases in two-dimensional materials

对称-电子指纹揭示二维材料中的竞争磁性相

Addis Fuhr, Zachary R. Fox, David Parker, Ayana Ghosh

AI总结 提出对称-电子指纹(SEF)表示,结合晶体对称性与电子结构,通过随机森林集成学习准确分类磁有序、回归磁矩和各向异性,并识别Stoner铁磁性与局域超交换的竞争区域,模型不确定性可诊断近简并铁磁/反铁磁相。

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AI中文摘要

二维磁体为自旋电子学和量子技术提供了引人注目的平台,但预测其磁基态、磁矩和各向异性仍然具有挑战性。这一限制主要源于现有的机器学习表示编码了化学环境,但没有捕捉控制磁性的对称性或交换物理。在这项工作中,我们引入了对称-电子指纹(SEF),这是一种物理可解释的表示,编码了晶体对称操作、Wyckoff位点几何以及位点分辨的电子结构。结合随机森林的集成学习,SEF在回归磁矩和各向异性能量的同时准确分类磁有序,同时分辨巡游Stoner铁磁性与局域超交换的不同区域。SEF训练模型的不同之处在于,模型不确定性较高的区域不是失败,而是一种诊断,识别出这些机制竞争的材料。对Co基和Ni基卤化物和氧化物的第一性原理计算证实,这些区域对应于具有磁受挫、抑制各向异性和涌现非共线有序的真正近简并FM和AFM相。通过将对称性和交换物理直接编码到表示中(不同于传统描述符),SEF将模型不确定性转化为指向二维材料的指南针,在这些材料中,小扰动驱动共线、受挫或非共线磁相之间的转变。

英文摘要

Two-dimensional magnets offer compelling platforms for spintronics and quantum technologies, yet predicting their magnetic ground states, moments, and anisotropy remains challenging. This limitation primarily arises because existing machine-learning representations encode chemical environments without capturing the symmetry or exchange physics that govern magnetism. In this work, we introduce the symmetry-electronic fingerprint (SEF), a physically interpretable representation that encodes crystallographic symmetry operations, Wyckoff-site geometry, together with site-resolved electronic structure. Combined with ensemble learning with random forests, the SEF accurately classifies magnetic ordering while regressing moments alongside anisotropy energies while simultaneously resolving the distinct regimes of itinerant Stoner ferromagnetism from localized superexchange. What sets the SEF-trained models apart is that regions of elevated model uncertainty are not a failure but a diagnostic, identifying materials where these mechanisms compete. First-principles calculations on Co- and Ni-based halides and oxides confirm that these regions correspond to genuine near-degenerate FM and AFM phases with magnetic frustration, suppressed anisotropy, and emergent non-collinear ordering. By encoding symmetry together with exchange physics directly into the representation unlike conventional descriptors, the SEF transforms model uncertainty into a compass pointing toward two-dimensional materials where small perturbations drive transitions between collinear, frustrated, or non-collinear magnetic phases.

2606.13541 2026-06-12 cond-mat.str-el cond-mat.supr-con 新提交

Overview of the Theory of Extremely Correlated Fermi Liquids

极端关联费米液体理论概述

B Sriram Shastry

AI总结 综述极端关联费米液体(ECFL)理论,用于理解接近Mott绝缘极限的金属系统中的t-J模型,并与单层高温超导体的电阻率和谱数据比较,揭示密度相关的准线性电阻、小准粒子权重和低温涌现尺度。

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AI中文摘要

极端关联费米液体(ECFL)理论被综述为一个框架,用于理解接近Mott绝缘极限的金属系统中的$t$-$J$模型。本概述以非专家可访问的形式呈现了基本思想和由此产生的方程。我们将理论结果与单层高温超导系统的所有可用电阻率数据以及一些谱数据进行了比较。突出的结果包括电阻率中密度依赖的准线性T依赖性、异常小的准粒子权重,以及主导单层高温超导体输运、热力学和谱性质的独特低温涌现尺度。提出了进一步实验的建议,以探索这些具有挑战性的量子多体系统的物理性质。

英文摘要

The Extremely Correlated Fermi Liquids (ECFL) theory is reviewed as a framework for understanding the $t$-$J$ model in metallic systems close to the Mott insulating limit. This overview presents the underlying ideas and the resulting equations in a form accessible to nonexperts. We compare theoretical results with all available resistivity data for single-layer High-T$_{c}$ systems, and with some spectral data. The highlighted results include a density dependent quasilinear T-dependence in resistivity, an unusually small quasiparticle weight, and distinct low-temperature emergent scales that dominate transport, thermodynamics and spectral properties of single-layer High T$_c$ systems. Suggestions are made for further experiments to probe the physics of these challenging quantum many-body systems.

2606.13540 2026-06-12 cond-mat.mes-hall physics.app-ph 新提交

Micron-sized magnonic 3-port rectilinear circulator

微米级磁振子三端口直线循环器

Kevin S. Weber, Loic Temdie, Vincent Castel, Timmy Reimann, Morris Lindner, Carsten Dubs, Yves Henry, Matthieu Bailleul, Vincent Vlaminck

AI总结 通过纳米线光栅手性激发自旋波,设计并实验验证了微米级三端口直线自旋波循环器,实现窄带可调谐(2-8 GHz)的非互易微波器件。

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Comments
10 pages, 4 figures, plus Appendix. Submitted to Physical Review Applied
AI中文摘要

与现代集成电路架构兼容的小型化非互易微波技术的发展仍然是现代信息技术的关键挑战。在这里,我们首次展示了微米级原型磁振子循环器的实验表征。利用通过纳米线光栅手性激发自旋波,我们提出了一种新颖的循环器设计,涉及三个直线和单向自旋波束通道。我们通过完整的3端口自旋波谱学证明了三个端口之间真正的自旋波循环。窄带工作频率可以在宽频率范围(2-8 GHz)内通过高达100 mT的外场以及指定波矢的光栅尺寸进行调谐。所提出的方案为集成和小型化非互易微波器件的新架构开辟了可能性。

英文摘要

The development of miniaturized non-reciprocal microwave technologies compatible with integrated circuit architectures remains a critical challenge for modern information technology. Here, we present the first experimental characterization of a micron-sized prototypical magnon circulator. Taking advantage of the chiral excitation of spin-waves via nanowire gratings, we propose an original design of a circulator involving three channels of rectilinear and unidirectional spin-wave beams. We demonstrate via a full 3-port spin-wave spectroscopy a genuine spin-wave circulation between the three ports. The narrow frequency band of operation can be tuned over a broad range of frequencies ($2$-$8$ GHz) with both an external field of up to $100$ mT, and the dimensions of the grating specifying the wavevectors. This proposed scheme opens up possibilities for new architectures of integrated and miniaturized non-reciprocal microwave devices.

2606.13534 2026-06-12 cond-mat.supr-con 新提交

Band-Selective Tunneling and Anisotropic Multiband Superconductivity in V$_2$Ga$_5$

V$_2$Ga$_5$中的带选择性隧穿和各向异性多带超导电性

Jozef Haniš, Jozef Kačmarčík, Filip Košuth, Levente Faber, Pavol Szabo, Szymon Królak, Michał J. Winiarski, Tomasz Klimczuk, Peter Samuely, Martin Gmitra

AI总结 通过热力学和光谱学结合第一性原理计算,揭示了V$_2$Ga$_5$中带选择性隧穿导致方向依赖的能隙层级反转,建立了各向异性多带s波配对模型。

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10 pages, 3 figures
AI中文摘要

具有结构各向异性的多带超导体为探索非常规量子态提供了肥沃的土壤,然而解析其方向性配对特性仍然是一个艰巨的挑战。在这里,我们对四方金属间化合物超导体$\text{V}_2\text{Ga}_5$($T_{\rm c} \approx 3.5$~K)进行了全面的热力学和光谱学研究,结合第一性原理电子结构计算与高灵敏度交流量热法和定向低温扫描隧道谱。通过在全对称$A_{1g}$表示中构建自洽的各向异性多带单重态$s$波配对模型,我们成功调和了实验比热和上临界场异常。关键的是,我们揭示了定向隧穿实验中体能隙层级反转的直接原因是带选择性隧穿。这一效应由局域费米速度“热点”与特定费米面拓扑之间的优雅相互作用主导,而非单纯的热力学能隙大小。我们的研究结果为高度单轴各向异性超导体中方向依赖的带选择性隧穿提供了清晰的微观图像,展示了方向依赖的输运约束如何塑造多带量子凝聚体的可观测特征。

英文摘要

Multiband superconductors with structural anisotropy offer a fertile ground for exploring unconventional quantum states, yet disentangling their directional pairing characteristics remains a formidable challenge. Here, we present a comprehensive thermodynamic and spectroscopic study of the tetragonal intermetallic superconductor $\text{V}_2\text{Ga}_5$ ($T_{\rm c} \approx 3.5$~K), combining first-principles electronic structure calculations with highly sensitive AC calorimetry and directional low-temperature scanning tunneling spectroscopy. By constructing a self-consistent, anisotropic multiband singlet $s$-wave pairing model within the fully symmetric $A_{1g}$ representation, we successfully reconcile the experimental specific heat and upper critical field anomalies. Crucially, we reveal that the apparent reversal of bulk gap hierarchies in directional tunneling experiments is a direct consequence of band-selective tunneling. This effect is governed by an elegant interplay between localized Fermi velocity 'hot spots' and specific Fermi surface topologies, rather than raw thermodynamic gap magnitudes alone. Our findings provide a clear microscopic picture of direction-dependent, band-selective tunneling in a highly uniaxial anisotropic superconductor, demonstrating how orientation-dependent transport constraints shape the observable signatures of multiband quantum condensates.

2606.13526 2026-06-12 cond-mat.supr-con 新提交

Quantum geometric anomalous Hall response in orbitally nonunitary superconductors

轨道非幺正超导体中的量子几何反常霍尔响应

Viktor Frilen, Annica M. Black-Schaffer, Ankita Bhattacharya

AI总结 本文研究多带超导体在光频下的反常霍尔响应,发现仅带内配对时,轨道非幺正性(而非自旋幺正性)通过量子几何效应产生有限响应,修正了超导体中Kerr信号的判据。

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6+6 pages, 3+1 figures
AI中文摘要

我们研究了多带超导体在光频下的反常霍尔响应(AHR),这一现象与极克尔效应密切相关,是超导体中时间反演对称性破缺的关键探针。在具有纯带内配对的平移不变多带系统中,伽利略不变性解耦了库珀对的质心和相对运动,导致普遍预期有限的AHR需要无序或有限的带间配对振幅。然而,这一限制可以通过多带布洛赫态固有的量子几何效应来解除。利用具有Kane-Mele自旋-轨道耦合的蜂窝晶格紧束缚模型,我们分析了仅带内配对的时间反演对称性破缺手性$d$波自旋单态和手性$p$波等自旋三重态配对态的AHR。通过解析和数值计算,我们证明自旋单态产生消失的AHR,即使其时间反演对称性破缺;而等自旋三重态表现出有限的AHR,即使它是自旋幺正的。我们将后者归因于轨道非幺正性,在自旋-轨道耦合存在下,它产生了有限AHR所需的自旋极化Bogoliubov准粒子态。该响应由量子几何决定的带间速度矩阵元介导。这一发现确立了自旋幺正但轨道非幺正的配对可以在没有带间配对的情况下产生有限的AHR,从而修正了超导体中Kerr信号的判据。

英文摘要

We investigate the anomalous Hall response (AHR) in a multiband superconductor at optical frequencies, a phenomenon intimately related to the polar Kerr effect, a key probe of time-reversal symmetry breaking in superconductors. In translationally invariant multiband systems with purely intraband pairing, Galilean invariance decouples center-of-mass and relative motion of Cooper pairs, leading to the widespread expectation that a finite AHR requires either disorder or finite interband pairing amplitudes. However, this restriction can be lifted by the quantum geometric effects inherent to multiband Bloch states. Using a honeycomb lattice tight-binding model with Kane-Mele spin-orbit coupling, we analyze the AHR for the time-reversal symmetry broken chiral $d$-wave spin-singlet and chiral $p$-wave equal-spin-triplet pairing states with intraband pairing only. We demonstrate, through both analytical and numerical calculations, that the spin-singlet state yields a vanishing AHR, even with its broken time-reversal symmetry, whereas the equal-spin triplet state exhibits a finite AHR, even when it is spin-unitary. We attribute the latter to orbital nonunitarity, which, in the presence of spin-orbit coupling, generates the spin-polarized Bogoliubov quasiparticle states required for a finite AHR. The response is mediated by interband velocity matrix elements governed by the quantum geometry. This finding establishes that spin-unitary, but orbitally nonunitary pairing, can generate a finite AHR even without interband pairing and thereby revises the criteria for Kerr signals in superconductors.

2606.13512 2026-06-12 cond-mat.supr-con physics.acc-ph 新提交

Current patterns and loss contributions in CORT cables carrying AC current

CORT电缆中交流电流的电流分布模式与损耗贡献

Benoît Vanderheyden, Julien Dular, Louis Denis, Steffen Elschner, Christophe Geuzaine, Mariusz Wozniak, Francesco Grilli

AI总结 本文通过有效二维模型研究单层CORT电缆中Garber电流分布对交流损耗的影响,揭示了表面损耗和边缘损耗的贡献机制。

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Comments
11 pages, 15 figures
AI中文摘要

导体绕管(CORT)电缆是在小截面中传输交流电的潜在解决方案。由于电缆的几何结构和涂层导体(CC)的螺旋排列,电流在每个CC内部遵循非平凡的模式。例如,对于单层电缆,电流主要沿CC外表面轴向流动,而沿内表面主要沿方位角方向流动。这种电流分布称为Garber电流模式,影响传输交流损耗。在数值模型中,通常采用的简化基于直导体或无限薄CC,这些方法忽略了Garber电流模式,从而错误地表示了CC内部的详细电流流动以及由此产生的三维场分布。本文研究了单层CORT电缆中CC的详细三维电流分布,作为电缆几何参数(如导体厚度、螺距角和相邻CC之间的间隙)的函数。特别地,研究了Garber电流模式对交流损耗的两个最大贡献的影响,即表面损耗(与平行于超导层宽面的磁场分量穿透相关)和边缘损耗(与CC间隙附近垂直磁场分量的穿透相关)。考察了CC中电流的详细分布,并建立了其与不同交流损耗机制的关系。本研究通过使用与电缆螺旋结构共形的坐标系的有效二维模型进行。

英文摘要

Conductor-on-round-tube (CORT) cables are a potential solution for carrying AC power in a small cross-section. Due to the geometry of the cable and the helical arrangement of the coated conductors (CC), the current follows a non-trivial pattern inside each CC. For instance, for the case of a single-layer cable, the current flow is mostly axial along the outer face of the CCs and mostly azimuthal along their inner face. Such a current distribution, known as the Garber current pattern, affects the transport AC losses. In numerical models, commonly adopted simplifications are either based on straight conductors or infinitely thin CCs. Such approaches neglect the Garber current pattern and thus misrepresent both the detailed current flow within the CC and the resulting 3D distribution of the fields. In this work, the detailed 3D current distribution in the CCs is investigated in a one-layer CORT cable, as a function of the cable geometrical parameters such as the conductor thickness, the pitch angle, and the gap between adjacent CCs. In particular, the impact of the Garber current pattern is studied on the two largest contributions to the AC losses, namely the surface losses (associated with the penetration of the component of the magnetic field parallel to the wide faces of the superconducting layer) and the edge losses (associated with the penetration of the perpendicular component of the magnetic field occurring in the vicinity of the gaps between the CCs). The detailed distribution of the currents in the CCs is examined and its relationship with the different AC loss mechanisms is established. This study is carried out by means of an effective 2D model that uses a system of coordinates conforming with the helical structure of the cable.

2606.13502 2026-06-12 cond-mat.quant-gas 新提交

Quasi-2D trapped tilted dipoles at zero and finite temperatures in the strongly dipolar regime

准二维陷阱中倾斜偶极子在强偶极子区域零温和有限温度下的研究

Juan Sánchez-Baena

AI总结 通过Bogoliubov理论研究准二维几何中完全极化偶极子在零温和有限温度下的行为,揭示倾斜角、粒子数和散射长度对系统的影响,并发现温度升高促进空间调制。

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Comments
14 pages, 11 figures
AI中文摘要

受最近在准二维几何中观察到偶极超固态条纹的实验[arXiv:2512.13280 (2025)]的启发,我们通过Bogoliubov理论研究了在强轴向约束几何中完全极化偶极子的陷阱系统,包括零温和有限温度。偶极子沿z轴受到强谐振陷阱,并在x-y平面内受到盒状陷阱。我们表征了陷阱系统在零温和有限温度下的物理性质,作为偶极子倾斜角、粒子数和散射长度的函数,并将自己限制在实验相关的大凝聚体分数区域。我们还展示了盒状陷阱的纵横比对系统液体特性及其结构的影响。我们观察到,在特定配置下,当温度升高而总粒子数保持不变时,空间调制显著增强,这与先前在3D几何中的蒙特卡洛结果定性一致。我们的结果有助于理解准二维极限和强偶极子区域中陷阱偶极系统的零温物理。此外,它们允许在实验相关条件下评估温度对其平衡性质的影响,这可能对测温应用有用。

英文摘要

Motivated by the recent experimental observation of dipolar supersolid stripes in a quasi two-dimensional geometry [ arXiv:2512.13280 (2025)], we study a trapped system of fully polarized dipoles in a strongly axially confined geometry, both at zero and finite temperatures, by means of Bogoliubov theory. The dipoles are strongly harmonically trapped along the z axis and subjected to a box trap in the x-y plane. We characterize the physics of the trapped system at zero and finite temperatures as a function of the tilting angle of the dipoles, the number of particles and the scattering length, restricting ourselves to the experimentally relevant regime of large condensate fractions. We also illustrate the influence of the aspect ratio of the box trap in the liquid character of the system and its structure. We observe a remarkable promotion of spatial modulations when temperature is increased while keeping the total particle number constant for specific configurations, in qualitative agreement with previous Monte Carlo results in a 3D geometry. Our results are useful to understand the zero temperature physics of the trapped dipolar system in the quasi-2D limit and in the strongly dipolar regime. In addition, they allow to assess the effect of temperature in its equilibrium properties in experimentally relevant conditions, which may be useful for thermometry applications.

2606.13500 2026-06-12 cond-mat.mes-hall cond-mat.stat-mech 新提交

Thermoelectric information engine driven by an autonomous Maxwell demon across quantum-to-classical transitions

由自主麦克斯韦妖驱动的热电信息引擎跨越量子到经典转变

Maximiliano Bernal Santibañez, Felipe Barra, Jose Mondaca

AI总结 研究三端热电引擎中量子相干和信息流的作用,通过双量子点与监测点构成自主麦克斯韦妖,识别两个量子-经典转变,并发现相干性可增强妖机制。

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AI中文摘要

我们研究了一个三端热电引擎,重点关注量子相干和信息流的作用。一个双量子点连接两个具有不同化学势的库,而第三个量子点通过库仑相互作用监测它们的占据状态,并可解释为自主麦克斯韦妖。在设备作为引擎运行的参数范围内,我们确定了这种解释成立的条件。系统动力学由Redfield主方程描述,使我们能够识别两个不同的动力学区域,其稳态由合适的Lindblad近似很好地捕捉。这两个区域定义了由量子点间隧穿强度控制的第一个量子-经典转变。我们进一步考虑了耦合到双量子点的声子浴的影响,该声子浴通过在小量子点间隧穿区域产生非相干输运和退相干,诱导了第二个量子-经典转变。我们确定了一个参数区域,其中声子诱导的退相干抑制了相干输运贡献和流向监测点的信息流,表明在该区域相干性可以增强妖机制。通过追踪这些交叉过程中的信息和输运性质,我们的模型展示了相干隧穿、退相干和非相干声子辅助输运如何在自主信息引擎中竞争,同时阐明了在每个区域中哪种热力学Lindblad描述是合适的。

英文摘要

We study a three-terminal thermoelectric engine, focusing on the role of quantum coherence and information flow. A double-dot connects two reservoirs at different chemical potentials, while a third dot monitors their occupation via Coulomb interaction and can be interpreted as an autonomous Maxwell demon. Within the parameter range where the device operates as an engine, we identify conditions under which this interpretation holds. The system dynamics is described within a Redfield master equation that allows us to identify two distinct dynamical regimes with steady states well captured by suitable Lindblad approximations. These two regimes define a first quantum-to-classical transition controlled by the interdot tunneling strength. We further consider the effect of a phonon bath coupled to the double-dot, which induces a second quantum-to-classical transition by generating incoherent transport and decoherence in the small interdot tunneling regime. We identify a parameter region where phonon-induced decoherence suppresses both the coherent transport contribution and the information flow toward the monitoring dot, suggesting that coherence can enhance the demon mechanism in this regime. By tracking information and transport properties across these crossovers, our model shows how coherent tunneling, decoherence, and incoherent phonon-assisted transport compete in an autonomous information engine, while clarifying which thermodynamic Lindblad description is appropriate in each regime.

2606.13498 2026-06-12 cond-mat.stat-mech math-ph physics.chem-ph 新提交

Population dynamics of surface-mediated autocatalytic processes

表面介导的自催化过程的种群动力学

Denis S. Grebenkov, Yilin Ye

AI总结 研究粒子在复杂环境中扩散至表面区域被杀死或复制的自催化过程,通过生成函数、矩分析和数值模拟揭示种群大小的长期行为。

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AI中文摘要

我们研究了表面介导的自催化过程的种群动力学,其中粒子在复杂环境中扩散到表面区域,在那里它们可以被杀死或复制。这些相反的机制相互竞争,导致种群规模的复杂随机演化。我们提供了种群大小生成函数的系统分析。我们还推导了其分布、均值、方差和高阶矩。为此,我们采用了几种等效描述,这些描述基于非线性积分方程和具有非线性边界条件的偏微分方程。我们检查了种群动力学在三种情况下的长期行为:平均种群大小消失、达到稳态水平或呈指数增长。底层积分方程的数值解和独立的蒙特卡洛模拟支持了我们的理论预测。

英文摘要

We investigate the population dynamics of surface-mediated autocatalytic processes, in which particles diffuse in a complex environment towards surface regions where they can be either killed or replicated. These opposite mechanisms compete with each other and lead to a sophisticated stochastic evolution of the population size. We provide a systematic analysis of the generating function of the population size. We also deduce its distribution, mean, variance and higher-order moments. For this purpose, we employ several equivalent descriptions of these quantities in terms of nonlinear integral equations and partial differential equations with nonlinear boundary conditions. We inspect the long-time behavior of the population dynamics in three regimes when the mean population size vanishes, reaches a steady-state level, or grows exponentially. A numerical solution of the underlying integral equations and independent Monte Carlo simulations support our theoretical predictions.

2606.13484 2026-06-12 cond-mat.soft 新提交

Tracking microscopic irreversibility during yielding of a colloidal fractal gel with Rheo-Echo-XPCS

利用Rheo-Echo-XPCS追踪胶体分形凝胶屈服过程中的微观不可逆性

William Chèvremont, Julien Bauland, Emmeline Brassac, Gonzalo Sanchez Vera, Stefano Aime, Frédéric Pignon, Thomas Gibaud

AI总结 通过引入流变回波X射线光子相关光谱(rheo-echo-XPCS),直接测量碳黑胶体分形凝胶在屈服过程中不可逆纳米尺度动力学,发现去相关速度与损耗正切成线性关系,并揭示结构从压缩指数到拉伸指数的演变。

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AI中文摘要

理解屈服过程中微观结构动力学与宏观力学响应之间的关系仍然是软物质物理中的一个核心挑战。本文介绍了流变回波X射线光子相关光谱(rheo-echo-XPCS),该技术采用与振荡剪切同步的非线性采集,能够直接测量应变幅度控制下不可逆的纳米尺度动力学。将其应用于碳黑胶体分形凝胶,我们在涡度方向强度自相关函数中解析出时间周期性的回波,其衰减编码了非仿射结构重排。我们发现:(i)在所有应变下,去相关呈弹道状,$\tau \propto q^{-1}$,其中去相关速度$v_\tau = 1/\langle q\tau \rangle$与损耗正切$\tan\delta = G''/G'$成线性关系,从而确立了$\tan\delta$作为不可逆结构去相关速率的直接宏观标志;(ii)函数形式从低应变下的压缩指数($\alpha \simeq 1.5$)连续演变为高应变下的拉伸指数($\alpha \simeq 0.5$),前者与完整网络中的三维偶极应变场一致,后者反映了在碎片化过程中应力传递从体相转移到准一维丝状骨架时维数从$d_f = 3$降至$d_f = 1$。

英文摘要

Understanding how microscopic structural dynamics relate to macroscopic mechanical response during yielding remains a central challenge in soft matter physics. Here, we introduce rheo-echo X-ray photon correlation spectroscopy (rheo-echo-XPCS) with nonlinear acquisition synchronized to oscillatory shear, enabling direct measurement of irreversible nanoscale dynamics under strain amplitude control. Applying this to a carbon black colloidal fractal gel, we resolve time-periodic echoes in the vorticity-direction intensity autocorrelation function whose decay encodes non-affine structural rearrangements. We find: (i)~ballistic-like decorrelation with $\tau \propto q^{-1}$ at all strains, where the decorrelation velocity $v_\tau = 1/\langle q\tau \rangle$ scales linearly with the loss tangent $\tan\delta = G''/G'$, establishing $\tan\delta$ as a direct macroscopic signature of the rate of irreversible structural decorrelation; (ii)~functional form continuous evolution from compressed exponential ($\alpha \simeq 1.5$) at low strain, consistent with three-dimensional dipolar strain fields in the intact network-to stretched exponential ($\alpha \simeq 0.5$) at high strain, reflecting a dimensional reduction from $d_f = 3$ to $d_f = 1$ as stress transmission shifts from bulk to quasi-one-dimensional filamentary backbones during network fragmentation.

2606.13483 2026-06-12 cond-mat.mes-hall physics.optics 新提交

Phonon polariton confinement in isotopically pure MOVPE-grown BN triangles

同位素纯MOVPE生长BN三角形中的声子极化子限制

Maximilian Scharpey, Oskar Schröer, Daniel Wigger, Lena Miler, Jakub Iwański, Andrzej Wysmołek, Johannes Binder, Iris Niehues

AI总结 利用MOVPE生长的同位素纯BN三角形,通过s-SNOM和nano-FTIR研究声子极化子,实现了长传播长度和可调谐限制模式,为纳米光子学和量子光学中的全外延微腔极化子谐振器铺平道路。

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AI中文摘要

声子极化子是由光和晶格振动共振杂化形成的准粒子,具有双曲色散等独特性质。在此背景下,剥离的六方氮化硼(hBN)已成为声子极化子研究的有前景材料。然而,为了推进实际应用,必须在大面积外延BN中展示高效的声子极化子传播和限制。针对这一问题,我们使用金属有机气相外延(MOVPE)生长的BN,并通过散射型扫描近场光学显微镜(s-SNOM)和纳米傅里叶变换红外光谱(nano-FTIR)研究声子极化子性质。我们报告了显著长的声子极化子传播长度,表明BN层的高晶体质量。通过使用外延生长的同位素纯三角形岛,我们进一步展示了高效的声子极化子限制,其模式图案可通过入射光波长调谐。我们的结果为实现用于纳米光子学和量子光学的全外延、微尺度、高质量极化子谐振器铺平了道路。

英文摘要

Phonon polaritons, quasiparticles formed by the resonant hybridization of light and lattice vibrations, exhibit unique properties like the possibility of hyperbolic dispersions. In this context, exfoliated hexagonal boron nitride (hBN) has emerged as a promising material for phonon polariton-based research. However, to advance toward practical applications, it is essential to demonstrate efficient phonon-polariton propagation and confinement in large-area epitaxial BN. To address this topic, we use metalorganic vapor phase epitaxy (MOVPE)-grown BN and investigate the phonon polariton properties using scattering-type scanning near-field optical microscopy (s-SNOM) and nanoscale Fourier transform infrared spectroscopy (nano-FTIR). We report remarkably long phonon polariton propagation lengths, indicating the high crystalline quality of the BN layer. By using epitaxially grown isotopically pure triangular islands, we further demonstrate efficient phonon-polariton confinement with mode patterns tunable by the incident light wavelength. Our results pave the way for implementing all-epitaxial, microscale, high-quality polariton resonators for nanophotonics and quantum optics.

2606.13424 2026-06-12 cond-mat.mtrl-sci 新提交

Dopant-induced modifications of the optical properties of GaSe

掺杂诱导的GaSe光学性质改性

Jakub Sójka, Katarzyna Olkowska-Pucko, Kacper Walczyk, Zakhar R. Kudrynskyi, Volodymyr Boledzjuk, Adam Babiński, Maciej R. Molas, Grzegorz Krasucki

AI总结 通过光致发光光谱研究Fe掺杂对GaSe光学性质的影响,发现Fe引入多种尖锐发射线并形成Fe束缚激子,磁光测量揭示两类g因子,表明Fe掺杂产生光学和磁性活性中心。

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Comments
6 pages, 4 figures + SI
AI中文摘要

掺杂在调控半导体的电子、光学和磁性质中起着关键作用,能够控制载流子动力学并形成用于光电子应用的功能态。我们利用变激发功率、温度和磁场下的光致发光(PL)光谱研究了Fe掺杂剂对GaSe晶体光学性质的影响。Fe的引入除了本征激子跃迁(包括自由激子和局域激子)外,还引入了多条尖锐的发射线。功率和温度依赖的测量表明,这些发射特征与Fe相关的掺杂剂中心(Fe束缚激子)有关。磁光PL测量揭示了两类不同的$g$因子,从而能够识别本征激子跃迁和Fe诱导的缺陷态。这些结果表明,Fe掺杂在GaSe中产生了光学和磁性活性中心,为缺陷相关的激子过程及其在磁光电子和量子光子应用中的潜在相关性提供了见解。

英文摘要

Doping plays a crucial role in tailoring the electronic, optical, and magnetic properties of semiconductors, enabling control of carrier dynamics and the formation of functional states for optoelectronic applications. We investigate the influence of Fe dopants on the optical properties of GaSe crystals using photoluminescence (PL) spectroscopy under varying excitation power, temperature, and magnetic field. Fe incorporation introduces multiple sharp emission lines in addition to intrinsic excitonic transitions, including free and localised excitons. Power- and temperature-dependent measurements indicate that these emission features are associated with Fe-related dopant centres (Fe-bound excitons). Magneto-PL measurements reveal two distinct families of $g$-factors, enabling the identification of intrinsic excitonic transitions and Fe-induced defect states. These results demonstrate that Fe doping creates optically and magnetically active centres in GaSe, providing insight into defect-related excitonic processes and their potential relevance for magneto-optoelectronic and quantum photonic applications.

2606.13420 2026-06-12 cond-mat.mtrl-sci 新提交

The phase composition and physical properties of melt-quenched multicomponent alloy FeCoNiB0.7Si0.3Be

熔淬多组元合金FeCoNiB0.7Si0.3Be的相组成与物理性质

Oleksandr I. Kushnerov, Sergey I. Ryabtsev, Pavlo O. Galagan, Valerij F. Bashev

AI总结 研究了高熵多组元合金FeCoNiB0.7Si0.3Be在铸态和熔淬态的结构与物理性质,发现熔淬态中B2相分数增加,微硬度降低,矫顽力显著增大。

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Comments
Accepted manuscript. 12 pages, 3 figures. Published in Functional Materials 32(3) (2025), 418-422. DOI: https://doi.org/10.15407/fm32.03.418
AI中文摘要

研究了高熵多组元合金FeCoNiB0.7Si0.3Be在铸态和熔淬态的结构与物理性质。基于薄膜厚度估算,熔淬薄膜的冷却速率约为10^6 K/s。X射线分析显示多相结构,包括BCC型有序相(结构类型B2)和金属间化合物(Fe, Ni, Co)2B。在熔淬样品中,B2相分数增加,导致微硬度从铸态的10400 MPa降至熔淬态的8900 MPa。磁性研究证实了FeCoNiB0.7Si0.3Be合金的铁磁性。熔淬样品的矫顽场(17500 A/m)显著高于铸态样品(5200 A/m),这归因于结构细化和微应力水平增加。

英文摘要

The structure and physical properties of the high-entropy multicomponent alloy FeCoNiB0.7Si0.3Be in the as-cast and melt-quenched states were studied. The cooling rate of the melt-quenched films was estimated to be approximately 10^6 K/s based on the film thickness. X-ray analysis revealed a multiphase structure, including a BCC-type ordered phase (structural type B2) and intermetallic compounds (Fe, Ni, Co)2B. In melt-quenched samples, the fraction of the B2 phase increased, leading to a decrease in microhardness from 10400 MPa in the as-cast state to 8900 MPa in the melt-quenched state. Magnetic studies confirmed the ferromagnetic nature of the FeCoNiB0.7Si0.3Be alloy. The coercive field of melt-quenched samples (17500 A/m) was significantly higher than that of the as-cast ones (5200 A/m), which is attributed to structure refinement and an increased level of microstresses.

2606.13414 2026-06-12 cond-mat.mtrl-sci 新提交

Physics-informed time-series forecasting of perovskite photoluminescence stability

钙钛矿光致发光稳定性的物理信息时间序列预测

Alexander Wieczorek (1), Manuel Kober-Czerny (1), Fábio Lopes (1), Austin George Kuba (2), Leon Müller (3), Christian M. Wolff (2), Jason Hattrick-Simpers (4,5), Sebastian Siol (1) ((1) Laboratory for Surface Science and Coating Technologies, Empa-Swiss Federal Laboratories for Materials Science and Technology, Dübendorf, Switzerland, (2) Institute of Electrical and Microengineering (IEM), Photovoltaic and Thin-Film Electronics Laboratory, EPFL -École Polytechnique Fédérale de Lausanne, Switzerland, (3) Fritz-Haber-Institut der Max-Planck-Gesellschaft, Berlin, Germany, (4) Department of Materials Science and Engineering, University of Toronto, Toronto, ON, Canada, (5) Acceleration Consortium, University of Toronto, Toronto, ON, Canada)

AI总结 提出一种物理信息时间序列预测算法,利用CNN-LSTM模型预测金属卤化物钙钛矿的长期光致发光稳定性,在167种材料上验证,优于基线方法并具有可解释性。

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Comments
The first three listed authors contributed equally to the manuscript
AI中文摘要

使用高温和光照加速老化是快速研究新型半导体材料稳定性的最常用方法之一。然而,随着材料发现速度的持续加快,需要更快的稳定性评估。本文提出了一种物理信息时间序列预测算法,旨在预测金属卤化物钙钛矿的长期光致发光稳定性。收集了167种金属卤化物钙钛矿的多样化实验数据集,包括不同的结晶度和组成。这些材料在热和光的作用下受到应力,同时监测光致发光(PL)。利用物理信息模型对收集的超过86k个PL光谱进行特征化,并训练混合CNN-LSTM模型来预测模型训练中未见过的样品在降解过程中的PL强度。值得注意的是,该方法在材料组间具有泛化能力,且优于基线基准。此外,基于物理的特征化确保了可解释性,能够分析识别给定预测的关键稳定性描述符。预计该方法将适用于其他类型的时间序列数据,并为显著减少实验测试时间提供途径。

英文摘要

Accelerated ageing using elevated temperatures and illumination is one of the most common methods to rapidly study the stability of novel semiconductor materials. However, as the pace of materials discovery continues to accelerate, even faster stability evaluations are needed. A physics-informed time-series forecasting algorithm designed to predict the long-term photoluminescence stability of metal halide perovskites is presented. A diverse experimental dataset of 167 metal halide perovskites is collected, including different crystallinities and compositions. These are stressed using heat and light, while the photoluminescence (PL) is monitored. The >86k collected PL spectra are featurized using a physics-informed model, and a hybrid CNN-LSTM model is trained to forecast the PL intensity during degradation of samples unseen during model training. Notably, the approach generalizes across the material groups and outperforms baseline benchmarks. Furthermore, the physics-based featurization ensures explainability, enabling analysis to identify critical stability descriptors for given predictions. It is expected that this approach will be adapted to other types of time-series data and enables a pathway to significantly reduce experimental testing times.

2606.13399 2026-06-12 cond-mat.mtrl-sci cond-mat.mes-hall 新提交

Enhanced Photocurrent Response in Epitaxial 0.5PZT-0.5PFN Multiferroic Thin Films

外延0.5PZT-0.5PFN多铁薄膜中增强的光电流响应

Lucia Imhoff, Miguel A. Rengifo, Jose M. Caicedo Roque, Jessica Padilla-Pantoja, Jose Santiso, Marcelo G. Stachiotti, Myriam H. Aguirre

AI总结 本研究通过脉冲激光沉积制备高度取向的0.5Pb(Zr0.52Ti0.48)O3-0.5Pb(Fe0.5Nb0.5)O3多铁薄膜,发现其具有良好铁电性和弱铁磁性,并展现出与极化相关的显著光电流响应,证实了铁电极化与光伏效应的内在耦合。

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AI中文摘要

探索具有铁电极化与光伏效应强耦合的新型多铁材料对于下一代光电器件至关重要。在本研究中,我们表征了通过脉冲激光沉积在具有SrRuO3底电极的SrTiO3 (001)衬底上生长的高度取向0.5Pb(Zr0.52Ti0.48)O3-0.5Pb(Fe0.5Nb0.5)O3多铁薄膜。薄膜表现出优异的结晶质量,具有单一钙钛矿相和(001)取向。它们显示出良好的铁电性能(剩余极化~17 μC/cm²,PUND;矫顽场~150 kV/cm),同时在室温下具有弱铁磁行为(剩磁1.30 emu/cm³;矫顽场90 Oe)。光伏测量表明,在403 nm单色激光照射下,具有稳健的、依赖于极化的光响应,Jsc值在±20 μA/cm²之间。这一引人注目的观察结果证实了铁电极化与光伏效应之间的内在耦合,突显了这些单相多铁薄膜在先进光伏和光电器件存储器应用中的巨大潜力。

英文摘要

The exploration of novel multiferroic materials with strong coupling between ferroelectric polarization and photovoltaic effects is crucial for next-generation optoelectronic devices. In this study, we characterized highly oriented 0.5Pb(Zr0.52Ti0.48)O3-0.5Pb(Fe0.5Nb0.5)O3 multiferroic thin films grown by pulsed laser deposition on SrTiO3 (001) substrates with a SrRuO3 bottom electrode. The films exhibited excellent crystalline quality, with a single perovskite phase and (001) orientation. They displayed good ferroelectric properties (remanent polarization $\sim$17 $\mu$C/cm$^2$, PUND; coercive field $\sim$150 kV/cm), alongside weak ferromagnetic behavior at room temperature (remanence 1.30 emu/cm$^3$; coercive field 90 Oe). Photovoltaic measurements demonstrated a robust, polarization-dependent photoresponse under 403 nm monochromatic laser illumination, achieving Jsc values between $\pm$20 $\mu$A/cm$^2$. This compelling observation confirms the intrinsic coupling between ferroelectric polarization and photovoltaic effects, highlighting the considerable promise of these single-phase multiferroic thin films for advanced photovoltaic and optoelectronic memory applications.

2606.13396 2026-06-12 cond-mat.mtrl-sci 新提交

Polarizing ultrathin ferroelectric BaTiO3 films through interfacial layer polarization

通过界面层极化实现超薄铁电BaTiO3薄膜的极化

Ipek Efe, Edith Simmen, Tobias Goldenberger, Manfred Fiebig, Nicola A. Spaldin, Morgan Trassin

AI总结 利用SmNiO3缓冲层的带电原子面作为极化模板,在超薄BaTiO3薄膜中稳定极化,并抑制了退极化场导致的临界厚度,实现了从第一个单胞开始出现净极化。

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AI中文摘要

将铁电薄膜集成到器件中的一个重要要求是在仅有几个单胞厚度的薄膜中确定性地控制极化状态。在这里,我们利用(001)取向的SmNiO$_3$ (SNO)缓冲层的带电原子面作为极化模板,来稳定铁电BaTiO$_3$ (BTO)模型系统薄膜中的极化。我们展示了通过选择[SmO]$^+$ ([NiO$_2$]$^-$)缓冲层终止面可以实现向上(向下)取向的极化。最重要的是,SNO的带电原子面抑制了BTO中由退极化场引起的临界厚度,并且我们记录到从沉积的第一个单胞开始,BTO薄膜中出现了净极化。我们的实验在密度泛函理论(DFT)计算的指导下,进一步强调了带电缺陷对SNO缓冲层极化效果的影响。具体来说,氧空位抵消了SNO缓冲层带负电的[NiO$_2$]$^-$终止面的极化场。我们的发现为理解缺陷化学与极化界面的相互作用提供了重要见解,从而将铁电极化稳定到单胞极限。

英文摘要

An important requirement for the integration of ferroelectric thin films into devices is deterministic control of the polarization state in films of only a few unit cells in thickness. Here, we utilize the charged atomic planes of (001)-oriented SmNiO$_3$ (SNO) buffer layers as a polarizing template to stabilize the polarization in ferroelectric BaTiO$_3$ (BTO) model system thin films. We show that an upwards (downwards) oriented polarization is achieved by selection of the [SmO]$^+$ ([NiO$_2$]$^-$) buffer termination. Most importantly, the charged atomic planes of SNO suppress the depolarizing-field-induced critical thickness in BTO, and we record the emergence of a net polarization in our BTO films from the first unit cell deposited. Our experiments, guided by density-functional-theory (DFT) calculations, further highlight the impact of charged defects on the polarizing effectiveness of the SNO buffer. Specifically, oxygen vacancies counteract the polarizing field of the negatively charged, [NiO$_2$]$^-$-terminated surface of the SNO buffer. Our findings provide important insights into the interplay of defect chemistry and polarizing interfaces to stabilize ferroelectric polarization down to the single-unit-cell limit.

2606.13395 2026-06-12 cond-mat.supr-con cond-mat.str-el 新提交

Andreev Reflection to Probe Momentum-Dependent Spin Polarization in Altermagnet CrSb

Andreev反射探测交变磁体CrSb中动量依赖的自旋极化

Yan Zhang, Yixuan Luo, Yue Yang, Zilong Li, Weilong Qiu, Lunhui Hu, Yuanfeng Xu, Yanfeng Guo, Chao Cao, Xin Lu

AI总结 利用超导Nb尖端的机械点接触谱测量CrSb单晶沿三个晶向的Andreev反射,提取出动量依赖的自旋极化率(73.4%、67.9%、61.9%),并观察到尺寸250-500 nm的交变磁畴,支持了交变磁体中动量依赖的自旋极化。

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Comments
7 pages, 5 figures
AI中文摘要

交变磁性材料最近作为下一代自旋电子学应用的有前途候选者出现,其特征是k依赖的自旋分裂能带结构和同时的零净磁化。其中,交变磁候选材料CrSb因其g波自旋分裂和高奈尔温度而引起了广泛关注。在本文中,我们使用带有超导Nb尖端的机械点接触谱(MPCS)沿三个主要晶向探测CrSb单晶上的Andreev反射。提取的动量依赖自旋极化率对于(0001)面约为73.4%,对于(-1-120)面约为67.9%,对于(10-10)面约为61.9%,这与传统的反铁磁体不同。此外,样品表面空间线扫描的电导谱支持存在特征尺寸为250-500 nm的交变磁畴,由宽度约250 nm的畴壁分隔。这些结果强烈支持交变磁体CrSb中的动量依赖自旋极化,并确立了Andreev反射作为探测k依赖自旋织构的新范式。

英文摘要

Altermagnetic materials have recently emerged as promising candidates for next-generation spintronic applications, characterized by the k-dependent spin-splitted band structure and a simultaneous zero-net-magnetization. Among them, altermagnetic candidate CrSb has attracted considerable attention, owing to its g-wave spin splitting and high Néel temperature. In this article, we employed mechanical point-contact spectroscopy (MPCS) with superconducting Nb tips to probe the Andreev reflection on CrSb single crystals along three principal crystallographic orientations. The extracted momentum-dependent spin polarizations are approximately 73.4% for the (0001) plane, 67.9% for the (-1-120) plane, and 61.9% for the (10-10) plane, respectively, distinct from conventional antiferromagnets. Furthermore, conductance spectra from spatial line-scans on the sample surface support the existence of altermagnetic domains with a characteristic size of 250-500 nm separated by domain-walls with width about 250 nm. These results strongly support the momentum-dependent spin polarization in altermagnetic CrSb and establish Andreev reflection as a new paradigm to probe k-dependent spin textures.