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2606.07178 2026-06-08 cond-mat.str-el 新提交

Phase diagram of the extended chequerboard $J-Q$ model

扩展棋盘格 $J-Q$ 模型的相图

Jiayou Yin, Lu Liu

AI总结 通过蒙特卡洛研究扩展棋盘格 $J-Q$ 模型的基态,发现仅存在从反铁磁态到plaquette单重态固态的直接一级相变,无中间相,且相变线呈现涌现 $O(4)$ 对称性。

Comments 9 pages, 17 figures

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AI中文摘要

棋盘格 $J-Q$ 模型被提出用于描述在 SrCu$_2({\rm BO}_3)_2$ 中观察到的从反铁磁(AFM)态到plaquette单重态(PS)固态的直接相变。本文中,我们对该模型的一个扩展版本的基态进行了蒙特卡洛研究。对于所有研究的参数,我们仅发现从AFM到PS相的直接一级相变,两者之间没有中间相。在相变线上,系统呈现出涌现的 $O(4)$ 对称性。此外,我们发现柱状价键固态的Binder比可用于定位相变。它表现出单调的有限尺寸标度行为,从而可以精确确定相变点。

英文摘要

The chequerboard $J-Q$ model was proposed to describe the direct phase transition from the antiferromagnetic (AFM) state to the plaquette-sin glet (PS) solid state observed in SrCu$_2({\rm BO}_3)_2$. In this paper, we present a Monte Carlo study of the ground state of an extended ve rsion of this model. For all parameters investigated, we find only a direct first-order phase transitions from the AFM to the PS phase, with no intermediate phase between them. On the transition line, the system exhibits an emergent $O(4)$ symmetry. Furthermore, we find that the Bi nder ratio of the columnar valence-bond solid state can be used to locate the phase transition. It exhibits a monotonic finite-size scaling b ehavior, allowing for a precise determination of the transition point.

2606.07138 2026-06-08 cond-mat.mtrl-sci 新提交

Chromium chalcohalide Janus monolayer ferromagnets with perpendicular magnetic anisotropy and high Curie temperature

具有垂直磁各向异性和高居里温度的铬硫卤化物Janus单层铁磁体

M. Bosnar, J. M. Lendinez, A. Yu. Vyazovskaya, I. Yu. Sklyadneva, R. Heid, S. V. Eremeev, U. Atxitia, S. Gallego, E. V. Chulkov, A. Arnau, M. M. Otrokov

AI总结 通过密度泛函理论,研究了非中心对称二维磁性材料铬硫卤化物单层CrXY(X=S, Se, Te; Y=Cl, Br, I)的磁性,发现1T相更稳定且所有动态稳定结构均显示铁磁耦合,其中CrSI和CrSeI具有垂直磁各向异性,并预测了高居里温度。

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Journal ref
Phys. Rev. B 113, 184425 (2026)
AI中文摘要

利用密度泛函理论,我们重新研究了最近提出的一类非中心对称二维磁性材料——铬硫卤化物单层CrXY(X=S, Se, Te; Y=Cl, Br, I)的磁性。这些系统由按X-Cr-Y序列堆叠的三个原子平面组成,破坏了反演对称性,因此被称为“Janus”单层。我们考虑了CrXY的1T和1H两种结构多型体。在这两种多型体中,1T相始终更稳定,每个化学式单元的能量增益超过0.55 eV。我们的总能量计算表明,所有动态稳定的CrXY单层均表现出铁磁耦合。然而,仅在CrSI和CrSeI组分中观察到稳健的面外磁各向异性,对于1T和1H结构均如此。垂直磁各向异性源于单离子各向异性和各向异性交换贡献之间的建设性相互作用,克服了偶极-偶极相互作用。我们进一步量化了CrSI和CrSeI中两种多型体的Dzyaloshinskii-Moriya相互作用(DMI),并揭示了与各向同性交换相互作用项相比,DMI强度为弱到中等。最后,对于表现出铁磁耦合和垂直磁各向异性的系统,将从密度泛函理论计算中得到的交换和各向异性参数作为输入,用于大规模原子自旋动力学模拟,以探测实空间磁结构的温度演化。计算得到的居里温度至少为:1T-CrSI 210 K,1H-CrSeI 235-260 K,1H-CrSI 370-410 K。相比之下,1T-CrSeI中显著的DMI导致在零外场下形成蠕虫状畴基态,并在垂直磁场下能够稳定斯格明子。

英文摘要

Using density functional theory, we revisit the magnetic properties of a recently proposed family of noncentrosymmetric two-dimensional magnetic materials, chromium chalcohalide monolayers, CrXY (X=S, Se, Te; Y=Cl, Br, I). These systems consist of three atomic planes stacked in the X-Cr-Y sequence, which breaks inversion symmetry, giving rise to their designation as "Janus" monolayers. We consider both 1T and 1H structural polymorphs of CrXY. Among the two polymorphs, the 1T phase is consistently more favorable, with energy gains exceeding 0.55 eV per formula unit. Our total-energy calculations reveal that all dynamically stable CrXY monolayers exhibit ferromagnetic coupling. However, robust out-of-plane magnetic anisotropy is observed only in the CrSI and CrSeI compositions, for both 1T and 1H structures. The perpendicular magnetic anisotropy results from a constructive interplay between single-ion and anisotropic exchange contributions that overcome the dipole-dipole interaction. We further quantify the Dzyaloshinskii-Moriya interaction (DMI) in CrSI and CrSeI for both polymorphs, and reveal a weak-to-moderate DMI strength as compared to the isotropic exchange interaction term. Finally, for systems exhibiting ferromagnetic coupling and perpendicular magnetic anisotropy, the exchange and anisotropy parameters derived from density functional theory calculations are employed as inputs for large-scale atomistic spin dynamics simulations to probe the temperature evolution of real-space magnetic structures. The calculated Curie temperatures are at least 210 K for 1T-CrSI, 235-260 K for 1H-CrSeI, and 370-410 K for 1H-CrSI. In contrast, the sizable DMI in 1T-CrSeI results in a worm-like domain ground state at zero external field and enables the stabilization of skyrmions under a perpendicular magnetic field.

2606.07137 2026-06-08 cond-mat.str-el 新提交

Inverse Melting of 3D Antiferromagnetic Order in Multi-sublattice Magnetic Perovskites

多子格磁性钙钛矿中三维反铁磁序的反向熔化

Bangye Qin, Dmitry D. Khalyavin, Ran Liu, Kazunari Yamaura, Alexei A. Belik, Roger D. Johnson

AI总结 通过中子粉末衍射发现,柱状有序四重钙钛矿NaRMn₂Ti₄O₁₂ (R = Dy, Sm)的基态缺乏长程有序,升温时先进入三维反铁磁有序再转变为顺磁态,揭示了由A位化学无序与稀土-Mn子格竞争交换耦合驱动的反常加热致有序机制。

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AI中文摘要

在常规反铁磁体中,长程有序的三维基态在升温时转变为无序顺磁态,通常通过临界区域内的低维自旋关联实现。在此,我们展示了与此范式截然不同的偏离。通过分析中子粉末衍射数据,我们表明柱状有序四重钙钛矿Na$R$Mn$_2$Ti$_4$O$_{12}$($R$ = Dy, Sm)的磁性基态缺乏长程有序,仅存在二维自旋关联。升温时,这一无序态在转变为顺磁态之前先转变为三维长程有序反铁磁结构。我们的结果建立了一种非常规的加热致有序机制,其中固有的A位化学无序与稀土和Mn子格之间的竞争交换相互作用耦合,导致了一种新型的磁性相变。

英文摘要

In conventional antiferromagnets a long-range ordered 3D ground state transitions to a disordered paramagnetic state on warming, often via lower dimensional spin correlations within the critical regime. Here we demonstrate a striking departure from this paradigm. Through analysis of neutron powder diffraction data, we show that the magnetic ground state of columnar-ordered quadruple perovskites, Na$R$Mn$_2$Ti$_4$O$_{12}$ ($R$ = Dy, Sm), lacks long-range order, hosting only 2D spin correlations. On warming, this disordered state transitions into a 3D long-range ordered antiferromagnetic structure prior to the phase transition to the paramagnetic state. Our results establish an unconventional order-by-heating mechanism in which intrinsic A-site chemical disorder is coupled to competing exchange interactions between the rare earth and Mn sub-lattices, leading to a novel type of magnetic phase transition.

2606.07133 2026-06-08 cond-mat.soft 新提交

Enhanced viscous adhesion using deformable structure

利用可变形结构增强粘附力

Mary Williams, Thomas Desmedt, Fabian Brau, Pascal Damman

AI总结 研究弹性薄结构与粘性流体接触并受控回缩时的粘附动力学,发现结构柔性引入强非线性力学响应,显著改变粘附力大小和演化,实现增强且可调的粘附。

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AI中文摘要

我们研究了薄弹性结构与粘性流体接触并以受控速度回缩时的粘附动力学,模拟了自然粘附机制。在分离过程中,可变形结构与刚性基底之间限制的粘性流体由于薄膜内的压降而产生粘附力。通过专门实验,我们发现结构柔性引入了强非线性力学响应,显著改变了粘附力的大小及其随回缩速度的演化。与刚性系统相比,结构的可变形性实现了增强且可调的粘附。为了捕捉这种相互作用,我们建立了一个耦合弹性和粘性的理论框架,为柔性结构如何实现粘附控制提供了新的见解。

英文摘要

We investigate the adhesion dynamics of a thin elastic structure in contact with a viscous fluid and retracted at a controlled speed, mimicking natural adhesion mechanisms. During detachment, the viscous fluid confined between the deformable structure and a rigid substrate generates an adhesive force due to a pressure drop within the thin film. We show from dedicated experiments that the structural flexibility introduces a strongly nonlinear mechanical response, which significantly alters both the magnitude and the evolution of the adhesion force with retraction velocity. In contrast to rigid systems, the deformability of the structure enables enhanced and tunable adhesion. To capture this interplay, we develop a theoretical framework that couples elasticity and viscosity, providing new insights into how flexible structures enable adhesion control.

2606.07112 2026-06-08 cond-mat.mtrl-sci 新提交

Skyrmions in Synthetic Antiferromagnets: Collapse and Nucleation

合成反铁磁体中的斯格明子:坍塌与成核

M. N. Potkina

AI总结 利用简化晶格模型,计算了合成反铁磁体中反铁磁束缚斯格明子对的坍塌和从钉扎反铁磁参考态成核的最小能量路径,揭示了坍塌的层序性及与成核的强不对称性。

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AI中文摘要

合成反铁磁体中的磁性斯格明子是有前景的纳米尺度比特,但其有用性取决于写入的斯格明子对能否可靠存活和产生。利用简化晶格模型,我们计算了反铁磁束缚斯格明子对坍塌以及从钉扎反铁磁参考态反向成核的最小能量路径。在反铁磁钉扎边界下,主鞍点能量随钉扎岛尺寸变化微弱,而斯格明子对最小能量则带有强烈的尺寸相关边界惩罚。对于大钉扎岛,坍塌是层序的,并且当该状态满足弛豫准则时,可以通过单层斯格明子中间态。在相同钉扎边界模型中,成核的逆向势垒远大于坍塌,显示出强不对称性,这与辅助层序写入一致。

英文摘要

Magnetic skyrmions in synthetic antiferromagnets are promising nanoscale bits, but their usefulness depends on how reliably a written pair survives and can be created. Using a reduced lattice model, we compute minimum energy paths for collapse of an antiferromagnetically bound skyrmion pair and for reverse nucleation from a pinned antiferromagnetic reference state. With antiferromagnetically pinned boundaries, the main saddle energy changes only weakly with pinned-island size, whereas the skyrmion-pair minimum carries a strong size-dependent boundary penalty. For large pinned islands, collapse is layer-sequential and can pass through a single-layer skyrmion intermediate whenever this state satisfies the relaxation criterion. The much larger reverse barrier for nucleation shows a strong asymmetry with collapse in the same pinned-boundary model and is consistent with assisted layer-sequential writing.

2606.07111 2026-06-08 cond-mat.quant-gas 新提交

Failure of the Quench Action Formalism for Mott Insulator Initial States

淬火作用形式对莫特绝缘体初态的失效

Garry Goldstein

AI总结 通过反例证明,对于莫特绝缘体初态与Lieb-Liniger气体本征态的重叠,淬火作用形式假设的平滑密度依赖性不成立,重叠具有高度奇异性。

Comments Comments are welcome

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AI中文摘要

淬火作用形式依赖于一个假设:一般初始态 $\left|\Psi_{0}\right\rangle $ 与可积模型本征态(通过快度 $\left|k_{1},...k_{N}\right\rangle $ 定义)的重叠可以写为:\begin{equation} \left\langle k_{1},...k_{N}\mid\Psi_{0}\right\rangle =\exp\left(-S_{\Psi_{0}}\left(\rho\left(k\right)\right)\right),\label{eq:Exponential} \end{equation} 其中 $\rho\left(k\right)$ 是态 $\left|k_{1},...k_{N}\right\rangle $ 的准粒子密度,$S_{\Psi_{0}}$ 是依赖于 $\Psi_{0}$ 的 $\rho\left(k\right)$ 的某个光滑函数。特别地,淬火作用形式假设重叠平滑地依赖于准粒子密度 $\rho\left(k\right)$。在这项工作中,通过显式反例,我们证明情况并非如此。我们考虑莫特绝缘体与Lieb-Liniger气体之间的淬火。我们证明,莫特绝缘体基态与Lieb-Liniger气体任意本征态的重叠具有高度奇异性,并且没有像式(1)这样的表达式适用。我们在Lieb-Liniger气体的Tonks-Girardeau极限下以及重叠的 $1/c$ 展开(其中 $c$ 是Lieb-Liniger气体的耦合常数)的领头阶进行证明。在附录中,我们展示了XXZ模型中与晶体态重叠的类似结果。

英文摘要

The quench action formalism relies on the assumption that the overlap between a generic initial state $\left|Ψ_{0}\right\rangle $ and an eigenstate of an integrable model - defined through the rapidities $\left|k_{1},...k_{N}\right\rangle $ - can be written as: \begin{equation} \left\langle k_{1},...k_{N}\midΨ_{0}\right\rangle =\exp\left(-S_{Ψ_{0}}\left(ρ\left(k\right)\right)\right),\label{eq:Exponential} \end{equation} where $ρ\left(k\right)$ is the quasiparticle density of the state $\left|k_{1},...k_{N}\right\rangle $ and $S_{Ψ_{0}}$ is some smooth function of $ρ\left(k\right)$ that depends on $Ψ_{0}$. In particular the quench action formalism assumes the overlap depends smoothly on the quasiparticle density $ρ\left(k\right)$. In this work, by explicit counter example, we show that this is not the case. We consider the quench between a Mott insulator and a Lieb Liniger gas. We show that the overlap between the ground state of the Mott insulator and arbitrary eigenstates of the Lieb Liniger gas has a highly singular behavior and no expression like Eq. (1) applies. We do so within the Tonks Girardeau limit of the Lieb Liniger gas and to leading order in the $1/c$ expansion for the overlap (with $c$ being the coupling constant of the Lieb Liniger gas). In the Appendix we show similar results for overlaps in the XXZ model with crystal states.

2606.07095 2026-06-08 cond-mat.mtrl-sci 新提交

Cocktail effect and robust Berry curvature driven anomalous Hall conductivity in the entropy-stabilized Heusler alloy Co$_2$(Ti$_{0.25}$V$_{0.25}$Cr$_{0.25}$Fe$_{0.25}$)Al

熵稳定Heusler合金Co$_2$(Ti$_{0.25}$V$_{0.25}$Cr$_{0.25}$Fe$_{0.25}$)Al中的鸡尾酒效应和稳健的贝里曲率驱动反常霍尔电导

Suraj Kushwaha, S. K. Panda, Sourav Marik, Kartik Samanta, Tirthankar Chakraborty

AI总结 本研究合成了熵稳定Heusler合金Co$_2$(Ti$_{0.25}$V$_{0.25}$Cr$_{0.25}$Fe$_{0.25}$)Al,通过实验和DFT计算证明其反常霍尔电导主要源于贝里曲率,且尽管存在化学无序,该电导仍与母体化合物相当,体现了鸡尾酒效应。

Comments 10 pages, 4 figures

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AI中文摘要

化学无序与贝里曲率驱动输运现象之间的相互作用仍然是熵稳定系统中一个重要的开放问题。在这里,我们合成了熵稳定的Heusler合金Co$_2$(Ti$_{0.25}$V$_{0.25}$Cr$_{0.25}$Fe$_{0.25}$)Al,并通过实验测量和密度泛函理论(DFT)计算相结合,系统地研究了其结构、磁性和磁输运性质。该体系结晶为立方空间群$Fm\Bar{3}m$,并表现出铁磁性,饱和磁化强度与Slater-Pauling预测高度一致。输运和磁输运测量揭示了金属行为和显著的反常霍尔效应,反常霍尔电导率约为$134.4~ \Omega^{-1}\cdot\text{cm}^{-1}$。结合实验观察和第一性原理计算,确定反常霍尔效应主要源于本征机制,源自电子能带的贝里曲率。值得注意的是,尽管存在显著的构型无序以及组成母体化合物的稀释,反常霍尔电导率仍与相应母体Heusler体系中报道的最大值相当。这种行为反映了鸡尾酒效应的体现,这是熵稳定系统的核心特征之一。我们的结果还表明,贝里曲率介导的输运在这种化学无序体系中持续存在,并指出熵工程可以成为调控本征反常霍尔响应的有前景的途径。

英文摘要

The interplay between chemical disorder and persistence of Berry curvature driven transport phenomena remains an important open question in entropy-stabilized systems. Here, we synthesize an entropy-stabilized Heusler alloy Co$_2$(Ti$_{0.25}$V$_{0.25}$Cr$_{0.25}$Fe$_{0.25}$)Al and systematically investigate its structural, magnetic, and magnetotransport properties using a combination of experimental measurements and density functional theory (DFT) calculations. The system crystallizes in cubic space group $Fm\Bar{3}m$ and exhibits ferromagnetism with saturation magnetization in close agreement with the Slater--Pauling prediction. Transport and magnetotransport measurements reveal metallic behavior and a pronounced anomalous Hall effect with an anomalous Hall conductivity of approximately $134.4~ Ω^{-1}$.cm$^{-1}$. Combined experimental observations and first-principles calculations establish that the anomalous Hall effect is predominantly intrinsic in origin and originates from the Berry curvature of the electronic bands. Remarkably, despite the substantial configurational disorder and the dilution of the constituent parent compounds, the anomalous Hall conductivity remains comparable to the largest values reported in the corresponding parent Heusler systems. This behavior reflects the manifestation of the cocktail effect, one of the core characteristics of entropy-stabilized systems. Our results also demonstrate that Berry curvature mediated transport persists in this chemically disordered system and indicates that entropy engineering can be a promising route for tuning intrinsic anomalous Hall responses.

2606.07002 2026-06-08 cond-mat.stat-mech nlin.CD 新提交

Phase lag enhances synchronization in coupled oscillators with inertia

相位滞后增强带惯性耦合振子的同步

Sudo Yi, Cook Hyun Kim, Heetae Kim, B. Kahng

AI总结 研究通过施加对称破缺相位滞后到部分振子,使主集群与高阶集群合并,从而增强带惯性二阶Kuramoto模型的全局同步。

Comments 7 pages, 3 figures

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AI中文摘要

带惯性的二阶Kuramoto模型表现出与无惯性一阶KM不同的动力学行为。一个核心差异是其同步性较低,因为出现了多个不同频率的同步集群。我们旨在研究如何通过向处于稳态的系统施加外部扰动(例如,对一部分振子施加对称破缺的相位滞后)来改善这种降低的同步性。我们发现,这种相位滞后引导主集群沿特定路径移动,使其能够与高阶集群合并,从而增强全局同步。我们的结果揭示了一种机制,通过该机制,受控的相位滞后可以改善惯性振子系统的同步,对惯性振子网络中的同步控制具有潜在意义。

英文摘要

The second-order Kuramoto model with inertia exhibits different dynamical behaviors than the first-order KM without inertia. A central difference is its lower synchronization due to the emergence of multiple synchronized clusters with different frequencies. We aim to investigate how such lowered synchronization can be improved by applying external perturbations to the system in a steady state, for example, a symmetry-breaking phase lag to a subset of oscillators. We find that this phase lag steers the primary cluster along a specific path and enables it to merge with higher-order clusters, thereby enhancing global synchronization. Our results reveal a mechanism by which controlled phase lag can improve entrainment in inertial oscillator systems, with possible implications for synchronization control in inertial oscillator networks.

2606.06999 2026-06-08 cond-mat.mes-hall quant-ph 新提交

Light-tunable quantum metric non-linear Hall response in Berry dipole semimetals

Berry偶极半金属中光可调量子度规非线性霍尔响应

Debashree Chowdhury, Awadhesh Narayan

AI总结 研究光对Berry偶极半金属中量子度规介导的非线性霍尔效应的影响,发现光可调谐量子度规偶极不对称性,并通过光振幅直接控制非线性响应方向。

Comments 6 Pages, 7 Figures

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AI中文摘要

我们研究了光对Berry偶极半金属中量子度规介导的本征非线性霍尔电导率的影响。我们发现,光诱导了量子度规非对角部分的可调不对称性,这表现为量子度规偶极的不对称性。我们表明,非线性响应可以直接通过光振幅进行调谐。特别地,我们注意到当光振幅超过阈值时,非线性霍尔信号的方向发生改变。因此,光成为控制拓扑半金属中量子几何响应的有前景的刺激手段。

英文摘要

We investigate the effect of light on quantum metric-mediated intrinsic nonlinear Hall conductivity in Berry dipole semimetals. We discover that light induces a tunable asymmetry in the off-diagonal part of the quantum metric, which is manifested by an asymmetry in the quantum metric dipole. We show that the nonlinear response can be tuned directly by the light amplitude. In particular, we note that the direction of the nonlinear Hall signal changes when the light amplitude is increased beyond a threshold value. Light thus emerges as a promising stimulus to control the quantum geometric response in topological semimetals.

2606.06992 2026-06-08 cond-mat.mtrl-sci 新提交

Iron-catalysed on-surface synthesis of substrate-decoupled graphdiyne monolayers

铁催化表面合成基底解耦石墨二炔单层

Alice Cartoceti, Simona Achilli, Gianni Conti, Eliecer Pelaez-Sifonte, Alessio Orbelli Biroli, Francesco Sedona, Paolo D'Agosta, Francesco Tumino, Andrea Li Bassi, Jorge Lobo-Checa, Carlo S. Casari

AI总结 通过添加微量铁原子,在Au(111)上成功合成了共价有序的石墨二炔单层,实现了结构解耦和约1.6 eV的带隙。

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AI中文摘要

石墨二炔构成了一类新兴的二维sp-sp2碳同素异形体,具有石墨烯无法实现的可调电子性质。尽管已尝试通过表面合成方案实现石墨二炔网络的无缺陷单层生长,但由于金属化中间体和反应副产物的持续存在,限制了长程共价有序所需的结构自组织,因此完全共价且结构有序的石墨二炔网络的实验实现仍然具有挑战性。在这里,我们证明在生长过程中向表面添加微量Fe原子可以显著改善Au(111)上共价二维石墨二炔单层框架的合成。通过低温扫描隧道显微镜和光谱学,结合密度泛函理论,我们揭示了反应的原子级表面动力学。我们展示了Fe原子的关键作用,它们与Br副产物键合,形成Fe-Br物种,促进Au吸附原子的去除,并在温和退火条件下驱动从金属化网络向纯共价框架的转化。此外,我们展示了共价石墨二炔网络在结构和电子上与底层金属基底解耦,显示出由p_z前沿轨道位置定义的约1.6 eV的有限带隙。这些结果为原子精确表面合成全碳石墨二炔建立了可行路线,并为补充石墨烯的半导体二维碳材料开辟了道路。

英文摘要

Graphdiynes constitute an emerging class of two-dimensional sp-sp2 carbon allotropes with tunable electronic properties not accessible by graphene. Although flawless monolayer growth of graphdiyne networks has been attempted by means of on-surface synthesis protocols, the experimental realization of fully covalent and structurally ordered graphdiyne networks remains challenging due to the persistence of metalated intermediates and reaction byproducts, limiting the structural self-organization required for long-range covalent order. Here, we demonstrate that adding minute amounts of Fe atoms on the surface during the growth can exceptionally improve the synthesis of a covalent 2D graphdiyne monolayer framework on Au(111). By means of low-temperature scanning tunneling microscopy and spectroscopy, combined with density functional theory, we unveil the atomic-scale surface dynamics of the reaction. We demonstrate the crucial role of Fe atoms that bond with Br by-products, thereby forming Fe-Br species that promote the removal of Au adatoms and drive the conversion from a metalated network to a purely covalent framework upon mild annealing conditions. Moreover, we show the covalent graphdiyne network to be structurally and electronically decoupled from the underlying metallic substrate, revealing a finite bandgap of about 1.6 eV defined by the position of p_z frontier orbitals. These results establish a viable route for the atomically precise on-surface synthesis of all-carbon graphdiynes, and open the way to semiconducting 2D carbon materials complementing graphene.

2606.06981 2026-06-08 cond-mat.stat-mech 新提交

Fate of the Ising universality class under nonreciprocal interactions

非互易相互作用下伊辛普适类的命运

M. Akritidis, A. Garcés, A. Vasilopoulos, M. Carosi, D. Levis, N. G. Fytas

AI总结 通过蒙特卡洛模拟和重整化群分析,研究二维伊辛模型在非互易视觉锥相互作用下的临界行为,发现非互易耦合虽不影响临界指数,但导致Binder累积量等无量纲量的各向异性偏离。

Comments 8 pages, 4 figures, 1 table, 2-page appendix

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AI中文摘要

我们研究了具有非互易视觉锥相互作用的二维伊辛模型的临界行为,这种相互作用明确违反了互易性和细致平衡。广泛的蒙特卡洛模拟和动态重整化群分析表明,在非互易耦合强度λ的广泛范围内,渐近临界指数与平衡伊辛普适类完全一致。相比之下,无量纲量如Binder累积量和关联长度比显示出明显的各向异性非平衡修正,并系统性地偏离其平衡伊辛值。重整化群流进一步表明,非互易扰动在Wilson-Fisher不动点处是不相关的,同时产生与λ^2成正比的临界温度的有限偏移。我们的结果证明了二维伊辛临界性对此类方向性相互作用的显著鲁棒性。

英文摘要

We study the critical behavior of a two-dimensional Ising model with nonreciprocal vision-cone interactions, which explicitly violate reciprocity and detailed balance. Extensive Monte Carlo simulations and dynamic renormalization-group analysis show that the asymptotic critical exponents remain fully consistent with the equilibrium Ising universality class over a broad range of nonreciprocal coupling strengths $λ$. In contrast, dimensionless quantities such as the Binder cumulant and the correlation-length ratio display pronounced anisotropic nonequilibrium corrections and systematically deviate from their equilibrium Ising values. The renormalization-group flow further demonstrates that the nonreciprocal perturbation is irrelevant at the Wilson-Fisher fixed point while generating a finite shift of the critical temperature proportional to $λ^2$. Our results demonstrate the remarkable robustness of two-dimensional Ising criticality against this class of directional interactions.

2606.06980 2026-06-08 cond-mat.mtrl-sci 新提交

Electric-field induced trends of exchange interactions in transition-metal trilayers

过渡金属三层膜中交换相互作用的电场诱导趋势

Moinak Ghosh, Stefan Heinze, Souvik Paul

AI总结 利用密度泛函理论,系统研究了外加电场下无支撑过渡金属三层膜中的海森堡对交换相互作用和超越海森堡的多自旋高阶交换相互作用,发现交换常数在低电场下呈线性变化,且高阶交换常数变化可达百分之十。

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AI中文摘要

利用密度泛函理论,我们在外加电场存在下,对无支撑过渡金属三层膜中的海森堡对交换相互作用和超越海森堡的多自旋高阶交换相互作用进行了系统研究。体系由夹在4$d$(Ru、Rh、Pd)和5$d$(Ir)过渡金属层之间的六方原子Fe层组成。考虑了4$d$覆盖层的fcc和hcp堆叠。为了扫描大部分磁相空间,我们计算了无电场和施加高达$\pm 1.0$ V/Å电场时自旋螺旋的能量色散。我们发现,施加电场后能量色散在定性上保持不变,磁基态不变。通过拟合能量色散得到的交换常数在电场高达约$\pm 0.6$ V/Å时表现出线性依赖。计算得到的对交换和高阶交换常数的符号在电场下保持不变,但其场致变化对4$d$覆盖层敏感。最近邻交换常数的变化在百分之几的量级,而次近邻交换常数的变化高达百分之几十。基于多$Q$态(如$uudd$态和3$Q$态)的总能计算了高阶交换常数。与对交换常数类似,我们发现高阶常数在低电场下几乎呈线性依赖,变化高达百分之十。我们研究了三个三层膜中电场的自旋相关屏蔽,并将对交换和高阶交换相互作用的变化与电场诱导的Fe局域态密度及其在费米能级处的变化联系起来。

英文摘要

Using density functional theory, we have performed a systematic study of the Heisenberg pairwise exchange interaction and the beyond Heisenberg multi-spin higher-order exchange interactions in unsupported transition-metal trilayers in the presence of external electric fields. The systems consist of a hexagonal atomic Fe layer sandwiched between 4$d$ (Ru, Rh, and Pd) and 5$d$ (Ir) transition-metal layers. Both fcc and hcp stacking of the 4$d$ overlayer has been taken into account. To scan a large part of the magnetic phase space, we have calculated the energy dispersion of spin spirals without and with applied electric fields up to $\pm 1.0$ V/Å. We find that the energy dispersion remains qualitatively the same upon applying the electric fields and the magnetic ground state remains unchanged. The exchange constants obtained by fitting the energy dispersions exhibit a linear dependence on the electric field up to values of about $\pm 0.6$ V/Å. The sign of the calculated pairwise and higher-order exchange constants remain unchanged with electric-field, however, their field induced variation is sensitive to the 4$d$ overlayer. The changes are on the order of a few percent for the nearest-neighbor exchange constant and up to a few ten percent for beyond nearest-neighbor constants. The higher-order exchange constants are calculated based on the total energies of multi-$Q$ states, such as the $uudd$ and the 3$Q$ state. Similar to the pairwise exchange constants, we find a nearly linear field dependence of the higher order constants at small electric fields and variations of up to ten percent. We study the spin-dependent screening of the electric field for the three trilayers and relate the modifications of the pairwise and higher-order exchange interactions to the electric field induced changes of the spin-dependent Fe local density of states and its variation at the Fermi level.

2606.06952 2026-06-08 cond-mat.mtrl-sci 新提交

Characterization of Nonlinear Dynamics in Semiconductors in Frequency Domain using Modulated Photoexcitation

利用调制光激发在频域中表征半导体中的非线性动力学

Attia Awan, Rong Tang, Zhou Kang, Khadga Jung Karki

AI总结 提出频域方法,通过分析相位调制光束诱导的光致发光频率分量,评估半导体中自由载流子和激子的复合速率等参数。

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AI中文摘要

半导体中的载流子动力学本质上是复杂的,因为存在不同激发物种(如自由载流子和激子)以及它们之间以及与陷阱和声子的相互作用。通常使用时间分辨响应来识别对动力学有贡献的过程。然而,响应通常是非指数的,导致解释上的歧义。在这里,我们提出了一种频域方法,以CdSe为测试系统,表征半导体中的非线性动力学。我们表明,通过分析由一对相位调制光束诱导的总光致发光中的频率分量,可以评估自由载流子和激子的不同类型复合速率等参数。该方法可用作表征与半导体器件功能相关的超快过程的简单诊断工具。

英文摘要

Carrier dynamics in semiconductors is inherently complex owing to the coexistence of different excited species, such as free carriers and excitons, and their interactions among themselves and with traps and phonons. It is usual to use time-resolved responses to identify the processes that contribute to the dynamics. However, the responses often are non-exponential, leading to ambiguity in the interpretation. Here, we propose a frequency domain method to characterize nonlinear dynamics in semiconductors using CdSe as the test system. We show that by analyzing the frequency components in the total photoluminescence induced by a pair of phase-modulated beams, the parameters, such as rates of different types of recombination of free carriers and excitons, can be evaluated. The method can be used as a simple diagnostic tool to characterize ultrafast processes that are relevant to the functionality of semiconductor devices.

2606.06948 2026-06-08 cond-mat.mes-hall 新提交

Spin SWAP operation in double quantum dots at the LaAlO3/SrTiO3 interface

LaAlO3/SrTiO3界面双量子点中的自旋SWAP操作

A. Sierant, J. Czarnecki, B. Szafran, P. Wójcik

AI总结 研究LaAlO3/SrTiO3界面双量子点中自旋SWAP操作,通过半经典和量子模拟分析自旋轨道耦合及轨道间耦合对自旋动力学的影响,揭示大量子点与小量子点中SWAP保真度的差异。

Comments 12 pages, 14 figures

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AI中文摘要

纳米尺度过渡金属氧化物异质结构制备的进展使这些平台成为实现自旋量子比特的有前途的候选者,主要得益于其电子结构的$d$特性,这可能导致超精细相互作用和自旋退相干的减少。在这里,我们系统研究了嵌入在LaAlO$_3$/SrTiO$_3$界面二维电子气中的双量子点内SWAP操作中的自旋控制。我们的分析从单电子自旋动力学研究开始,重点关注自旋轨道耦合和轨道间耦合对自旋演化的影响。在这种情况下,我们的发现得到了基于布洛赫方程的半经典计算的支持,该计算与全量子力学模拟显示出良好的一致性。然后,我们通过分析两个区域之间的交叉来模拟SWAP操作:(i) 大量子点,其中电子结构由$d_{xy}$轨道主导,自旋动力学主要受Rashba型自旋轨道相互作用影响;(ii) 小量子点,其中更高能量的$d_{xz/yz}$轨道对电子结构有贡献,导致SWAP保真度显著降低。在第一个区域中,从应用角度来看特别相关,我们详细分析了由自旋轨道耦合引起的SWAP操作的各向异性。

英文摘要

Progress in the fabrication of nanoscale transition-metal-oxide heterostructures makes these platforms promising candidates for the realization of spin qubits, mainly due to the $d$-character of their electronic structures, which could potentially result in a reduction of hyperfine interactions and spin decoherence. Here, we present a systematic study of spin control within the SWAP operation in double quantum dots embedded in a two-dimensional electron gas at the LaAlO$_3$/SrTiO$_3$ interface. Our analysis starts with a study of single-electron spin dynamics, focusing on the influence of spin-orbit and interorbital coupling on the spin evolution. In this case, our findings are supported by semiclassical calculations based on the Bloch equations, which show good agreement with full quantum mechanical simulations. We then simulate the SWAP operation by analyzing the crossover between two regimes: (i) large quantum dots, where the electronic structure is dominated by the $d_{xy}$ orbitals and the spin dynamics is affected primarily by Rashba-type spin-orbit interaction; and (ii) small quantum dots, where higher-energy orbitals $d_{xz/yz}$ contribute to the electronic structure, leading to a significant reduction in the SWAP fidelity. In the first regime, particularly relevant from the application point of view, we analyze in detail the anisotropy of the SWAP operation induced by the spin-orbit coupling.

2606.06939 2026-06-08 cond-mat.mes-hall 新提交

Layer-Polarization-Driven Metal-Insulator Transition in multi-band Graphene Moire' Superlattices

多层石墨烯莫尔超晶格中层极化驱动的金属-绝缘体相变

Harsimran Kaur Mann, Simrandeep Kaur, Harsimran Singh, Yashashwani Garg, Amogh Waghmare, Mohit Kumar Jat, Kenji Watanabe, Takashi Taniguchi, Manish Jain, Aveek Bid

AI总结 通过垂直位移场调控层极化,在ABA堆叠三层石墨烯/hBN莫尔超晶格中实现从多带到单带的能带重构,并观测到空穴掺杂次级狄拉克点处的金属-绝缘体相变,量子电容测量和理论计算证实了带隙打开和层选择性耦合机制。

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AI中文摘要

石墨烯/hBN莫尔超晶格为探索低维系统中的涌现量子相提供了一个高度可调的平台。在这里,我们研究了hBN与ABA堆叠三层石墨烯(TLG)形成的莫尔超晶格,这是一个固有的多带系统。我们证明莫尔势不仅是一种微扰,更是杂化TLG中不同无质量和有质量电子能带的工具。通过施加垂直位移场来调控层极化,我们驱动了电子能带结构的基本重构。具体来说,增加位移场使系统从低能下的多带区域演变为有效的单带区域,伴随着空穴掺杂次级狄拉克点处的金属-绝缘体相变。这种相变源于载流子在石墨烯层间的重新分布,选择性地增强了它们与外禀莫尔势的耦合。量子电容测量为空穴侧次级狄拉克点处态密度的抑制提供了直接证据,这与带隙打开和位移场调控带隙的出现一致。理论计算重现了这些观测结果,并确定了层选择性耦合到莫尔势是潜在的机制。这些结果展示了在低维莫尔系统中对涌现绝缘相的电学控制,并强调了多带莫尔异质结构中的层极化和层选择性耦合通过能带结构重构和电子相互作用为工程拓扑和关联相提供了强大途径。

英文摘要

Graphene/hBN moiré superlattices provide a highly tunable platform for exploring emergent quantum phases in low-dimensional systems. Here, we investigate the moiré superlattice formed between hBN and ABA-stacked trilayer graphene (TLG), an inherently multi-band system. We demonstrate that the moiré potential is not merely a perturbation but a tool to hybridize the distinct massless and massive electronic sectors of TLG. By applying a perpendicular displacement field to tune layer polarization, we drive a fundamental reconstruction of the electronic band structure. Specifically, increasing the displacement field evolves the system from a multi-band regime to an effectively single-band regime at low energies, accompanied by a metal--insulator transition at the hole-doped secondary Dirac point. This transition originates from a redistribution of carriers across graphene layers that selectively enhances their coupling to the extrinsic moiré potential. Quantum capacitance measurements provide direct evidence for the suppression of the density of states at the hole-side secondary Dirac point, consistent with gap opening and the emergence of a displacement-field-tuned band gap. Theoretical calculations reproduce these observations and identify layer-selective coupling to the moiré potential as the underlying mechanism. These results demonstrate electrical control of an emergent insulating phase in a low-dimensional moiré system, and highlight that layer polarization and layer-selective coupling in multi-band moiré heterostructures provide a powerful route for engineering topological and correlated phases through band structure reconstruction and electron interactions.

2606.06925 2026-06-08 cond-mat.stat-mech cond-mat.dis-nn 新提交

A Machine-Learning Based Approach to the Evaluation of the Critical Scaling Behavior of Anisotropic Spin Systems

基于机器学习的方法评估各向异性自旋系统的临界标度行为

Alina A. Chubarova, Ivan A. Mamonov, Marina V. Mamonova, Mikhail I. Bogachev, Pavel V. Prudnikov

AI总结 提出基于卷积神经网络的机器学习方法,从蒙特卡罗模拟的相关矩阵中识别各向异性自旋系统的临界点,以多种方式提取临界温度,计算成本降低约10倍。

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AI中文摘要

能够充分表示相变并评估关键系统参数的计算模型对于理解各种材料的性质至关重要。这里我们提出一种基于机器学习的方法来识别各向异性自旋系统中的临界点。我们的方法包括从蒙特卡罗模拟获得的相关矩阵训练卷积神经网络模型。接下来,预训练模型被用作临界温度的快速估计器,可以通过几种互补的方式从CNN模型推理中提取临界温度,从而提高分析的鲁棒性。本研究中获得的基于机器学习的估计与参考蒙特卡罗模拟结果非常一致,而计算成本相比经典热力学方法降低了约10倍。

英文摘要

Computational models adequately representing phase transitions and evaluating the critical system parameters are essential for the understanding of the properties of a wide range of materials. Here we propose a machine learning (ML)-based approach to the identification of the critical point in anisotropic spin systems. Our approach implies training of a convolutional neural network (CNN) model from the correlation matrices obtained by Monte Carlo simulations. Next, the pretrained model is employed as a fast estimator of the critical temperature, which can be extracted in several complementary ways from the CNN model inference, this way improving the robustness of the analysis. The ML-based estimates obtained in this study are in very good agreement with the reference Monte Carlo simulation results, while computational costs are about 10x lower compared to the classical thermodynamic approach.

2606.06874 2026-06-08 cond-mat.stat-mech 新提交

Impact of capacity volatility and input substitutability on supply chain resilience

容量波动性与投入替代性对供应链韧性的影响

Jaeseok Hur, Juha Jang, Meesoon Ha, Hawoong Jeong

AI总结 基于Feld-Barthelemy框架,研究容量波动性和投入替代性如何通过截断正态分布和修正Leontief生产函数影响供应链韧性,发现降低波动性和结构多样化比增加平均容量更有效。

Comments 8 pages, 4 figures in the main text, and 3 figures in the appendices

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AI中文摘要

供应链由于其顺序生产依赖性,本质上容易受到随机冲击的影响。基于Feld-Barthelemy框架,我们研究了容量波动性和投入替代性如何决定随机供应链中的关键需求。通过使用截断正态分布对生产能力进行建模,我们表明在长供应链中,降低容量波动性通常比增加平均容量更有效,强调了企业层面同步的必要性。此外,引入修正的Leontief型生产函数揭示,投入替代性有效地分散了随机冲击。供应商多样化即使是在固定最大容量下,也通过引入网络拓扑效应独立增强了实物库存的韧性,从而固有地提高了关键需求。我们的发现表明,缓解容量波动性和结构性地多样化供应路线对于供应链韧性与传统的库存扩张同样至关重要。

英文摘要

Supply chains are intrinsically vulnerable to stochastic shocks due to their sequential production dependencies. Building on the Feld-Barthelemy framework, we investigate how capacity volatility and input substitutability determine critical demands in stochastic supply chains. By modeling production capacity with a truncated normal distribution, we show that in long supply chains, reducing capacity volatility is often more effective than increasing average capacity, emphasizing the need for firm-level synchronization. Furthermore, introducing a modified Leontief-type production function reveals that input substitutability effectively disperses stochastic shocks. Supplier diversification inherently raises critical demands, even under fixed maximum capacities, by introducing the effect of network topology that independently enhances the resilience of physical stock. Our findings demonstrate that mitigating capacity volatility and structurally diversifying supply routes are just as crucial to supply chain resilience as traditional inventory expansion.

2606.06858 2026-06-08 cond-mat.str-el 新提交

Complex Temperature-dependent Thermal Conductivity in a Sawtooth Chain Magnet Fe$_\mathrm{2}$SiSe$_\mathrm{4}$

锯齿链磁体Fe$_\mathrm{2}$SiSe$_\mathrm{4}$中与温度相关的复杂热导率

Kunya Yang, Feihao Pan, Liran Wang, Chenglin Shang, Ying Zhu, Xiancai Hu, Sanjiang He, Xinrun Mi, Long Zhang, Aifeng Wang, Yisheng Chai, Frederic Hardy, Christoph Meingast, Peng Cheng, Mingquan He

AI总结 通过热输运测量研究锯齿三角晶格橄榄石磁体Fe$_2$SiSe$_4$中自旋-声子耦合导致的双峰热导率结构,发现低温峰比高温峰增强约5倍。

Comments 10 pages, 3 figures

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Journal ref
Phys. Rev. B 113, 174442(2026)
AI中文摘要

几何阻挫磁体为探索晶格几何与自旋自由度之间的相互作用提供了理想平台。本文通过热输运测量研究了三角锯齿晶格橄榄石磁体Fe$_\mathrm{2}$SiSe$_\mathrm{4}$中晶格与自旋的相互作用,该材料在$T_1 = 110$ K(反铁磁)和$T_2 = 50$ K(亚铁磁)处发生连续磁相变。尽管热导率由声子主导,但其温度依赖性显示出由自旋-声子耦合引起的显著双峰结构。在$T_1$和$T_2$之间的中间温度范围内,声子被约5 meV的磁激发共振散射,在60 K附近产生一个宽峰。在$T_2$以下,共振自旋-声子散射被强烈抑制,导致热导率在冷却时迅速增加,并在11 K附近出现一个明显的低温峰,这是由传统声子散射机制控制的热输运特征。值得注意的是,该低温峰比高温宽峰增强了约5倍。这些结果表明热输运对自旋-晶格相互作用的高度敏感性,并突显自旋-声子散射是调控几何阻挫磁体中热导率的有效机制。

英文摘要

Geometrically frustrated magnets provide an ideal platform for exploring the interplay between lattice geometry and spin degrees of freedom. Here, we investigate the interactions between lattice and spin via thermal-transport measurements on the triangular sawtooth-lattice olivine magnet Fe$_\mathrm{2}$SiSe$_\mathrm{4}$, which exhibits successive magnetic transitions at $T_1 = 110$ K (antiferromagnetic) and $T_2 = 50$ K (ferrimagnetic). Although phonons dominate the thermal conductivity, its temperature dependence displays a pronounced double-peak structure arising from spin-phonon coupling. In the intermediate temperature range between $T_1$ and $T_2$ , resonant scattering of phonons by magnetic excitations around 5 meV produces a broad maximum around 60 K. Below $T_2$, the resonant spin-phonon scattering is strongly suppressed, leading to a rapid increase in thermal conductivity upon cooling and a pronounced low-temperature peak near 11 K, characteristic of heat transport governed by conventional phonon scattering mechanisms. Notably, this low-temperature peak is enhanced by a factor of $\sim 5$ compared to the broad maximum at higher temperatures. These results demonstrate the strong sensitivity of thermal transport to spin-lattice interactions and highlight spin-phonon scattering as an effective mechanism for tailoring thermal conductivity in geometrically frustrated magnets.

2606.06771 2026-06-08 cond-mat.mtrl-sci 新提交

Atomic-scale phase-field modeling for 2D ferroelectrics including non-Gaussian fluctuations

包含非高斯涨落的二维铁电体原子尺度相场建模

Kairi Masuda, Yu Kumagai

AI总结 通过引入非高斯涨落扩展原子尺度相场模型,应用于单层SnTe,准确预测极化与铁电-顺电相变,并揭示Sn原子熵贡献驱动相变。

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AI中文摘要

原子尺度相场建模通过将原子振动的概率密度视为场变量,并利用该原子场与原子间势构建相应的自由能泛函,将相场框架扩展到单个原子水平。通过这种方式,该框架有潜力以原子级分辨率可视化局部热力学状态,正如传统相场建模在介观尺度上作为自由能、应力及相关量的计算显微镜一样。然而,现有公式主要假设原子振动服从高斯概率分布,这限制了其在更复杂和异质系统(如表面)中的适用性。在本工作中,我们通过扩展自由能泛函以包含非高斯涨落,推广了原子尺度相场方法。我们将该方法应用于NVT系综中的单层SnTe,并表明预测的平衡极化与分子动力学模拟更吻合,且成功再现了铁电-顺电相变。此外,通过按原子分解熵,我们可视化了局域熵的原子分辨图,并发现高温下Sn原子对熵的贡献强于Te原子,这是铁电-顺电相变的驱动因素。这些结果拓宽了相场方法在更广泛原子系统中的应用,并为基于高分辨率热力学的原子分辨相变理论提供了途径。

英文摘要

Atomic-scale phase-field modeling extends the phase-field framework down to the level of individual atoms by treating the probability density of atomic vibrations as a field variable and constructing a corresponding free-energy functional from this atomic field together with interatomic potentials. In this way, the framework has the potential to visualize local thermodynamic states with atomic-level resolution, just as conventional phase-field modeling has served as a computational microscope for free energy, stress, and related quantities at mesoscopic scales. However, existing formulations mainly assume Gaussian probability distributions for atomic vibrations, which limits their applicability to more complex and heterogeneous systems such as surfaces. In this work, we generalize the atomic-scale phase-field methodology by extending the free-energy functional to include non-Gaussian fluctuations. We apply this approach to monolayer SnTe in the NVT ensemble and show that the predicted equilibrium polarization is in better agreement with molecular dynamics simulations and that the ferroelectric-to-paraelectric phase transition is successfully reproduced. Furthermore, by decomposing the entropy on a per-atom basis, we visualize atomically resolved maps of local entropy and find that Sn atoms contribute more strongly to the entropy than Te atoms at high temperature, which is a driving factor of the ferroelectric-to-paraelectric phase transition. These results broaden the applicability of phase-field approaches to a wider range of atomic systems and suggest a route toward an atom-resolved theory of phase transitions based on high-resolution thermodynamics.

2606.06734 2026-06-08 cond-mat.mtrl-sci 新提交

Engineering magnetic anisotropy and ferromagnetism in topological Kagome metal GdV6Sn6 via Nd substitution

通过Nd替代调控拓扑Kagome金属GdV6Sn6的磁各向异性和铁磁性

Santosh Karki Chhetri, M. M. Sharma, Jian Wang, Dinesh Upreti, Gokul Acharya, Md Rafique Un Nabi, Jin Hu

AI总结 本研究通过Nd替代Gd,将Kagome金属GdV6Sn6的复杂磁基态调控为类铁磁态,并引入磁各向异性,揭示了稀土替代在调控磁性和磁输运行为中的作用。

Comments 25 pages, 6 figures

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Journal ref
Physical Review B 113,224417(2026)
AI中文摘要

具有化学式RM6X6(R=稀土,M=3d过渡金属,X=Sn/Ge)的Kagome金属为探索磁性和电子现象提供了丰富平台,其可调性质得益于稀土元素和过渡金属的组合。在本研究中,我们报道了Kagome金属(NdxGd1-x)V6Sn6的结构、电学和磁学性质。我们证明,在Gd位点替代较轻的Nd原子可将GdV6Sn6的复杂磁基态调控为类铁磁态。此外,GdV6Sn6的各向同性磁化变为各向异性,c轴成为易轴。输运测量揭示了磁性与电子性质之间的强耦合,在所有组分中低磁场下均观察到负磁电阻。另外,在端元化合物中,高磁场下倾向于出现四重各向异性分量。这些发现突显了稀土替代在调控具有非磁性Kagome层的RM6X6化合物中磁各向异性和磁输运行为的作用,对自旋电子学和拓扑应用具有潜在意义。

英文摘要

Kagome metals with the formula RM6X6 (R = rare-earth, M = 3d transition metal, and X = Sn/Ge) provide a rich platform for exploring magnetic and electronic phenomena, with tunable properties enabled by the combination of rare-earth elements and transition metals. In this study, we report the structural, electrical and magnetic properties of Kagome metal (NdxGd1-x)V6Sn6. We demonstrate that substituting lighter Nd atoms at the Gd site tunes the complex magnetic ground state of GdV6Sn6 into a ferromagnetic-like one. Moreover, the isotropic magnetization of GdV6Sn6 becomes anisotropic, with the c-axis emerging as the easy axis. Transport measurements reveal a strong coupling between magnetism and electronic properties, with negative magnetoresistance observed at low magnetic fields in all compositions. In addition, a fourfold anisotropy component tends to emerge in end compounds at higher magnetic fields. These findings highlight the role of rare-earth substitution in tuning magnetic anisotropy and magneto-transport behaviour in RM6X6 compounds, featuring a non-magnetic Kagome layer, with potential implications for spintronic and topological applications.

2606.06716 2026-06-08 cond-mat.dis-nn cond-mat.mes-hall 新提交

Persistent currents in signed directed networks

有符号有向网络中的持续电流

Davide Cipollini, Guido Caldarelli

AI总结 将有符号磁拉普拉斯算子解释为有效哈密顿量,在任意拓扑网络中定义持续电流,揭示量子相干性与循环空间几何的直接关联。

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AI中文摘要

网络理论可有效描述物理系统中的量子相干性。为此,我们将有符号磁拉普拉斯算子解释为有效哈密顿量,并将关联的边相位视为离散规范场,从而在有符号有向网络中引入持续电流。在正则系综中,持续电流作为规范不变通量变化的热力学响应出现。我们证明这些通量自然定义在网络循环空间上,且产生的电流被约束在无散子空间中并分解为独立循环。该公式将持续电流从环和晶格直接推广到任意拓扑。持续电流的检测提供了网络支持的量子相位相干的标志,以及其循环空间几何的直接标志。这种映射不仅为量子技术领域中多种情况的量子相干性处理提供了实用方法,还允许对图论中拉普拉斯算子的重要性进行物理解释,将其作用与物理系统中的哈密顿量(即紧束缚哈密顿量)联系起来。为测试该方法的能力,我们构建了一个重现霍夫施塔特蝴蝶谱的有符号有向网络。

英文摘要

Network theory can be fruitfully used to describe quantum coherence in physical systems. To that purpose we introduce persistent currents in signed directed networks by interpreting the signed magnetic Laplacian as an effective Hamiltonian and the associated edge phases as a discrete gauge field. In a canonical ensemble, persistent currents arise as thermodynamic responses to variations of gauge-invariant fluxes. We show that these fluxes are naturally defined on the cycle space of the network, and that the resulting currents are constrained to the divergence-free subspace and decompose onto independent cycles. This formulation provides a direct generalization of persistent currents from rings and lattices to arbitrary topologies. Detection of persistent currents provides a signature of the quantum phase coherence supported by the network, and a direct signature of the geometry of its cycle space. Such a mapping, not only allows a practical way to deal with quantum coherence for a variety of situations in the field of quantum technologies, but it also allows a physical interpretation of the importance of the Laplacian operator in graph theory, linking its role to the one of Hamiltonian (i.e. a tight-binding one) in physical systems. To test the power of the method, we construct a signed directed network that reproduces the Hofstadter butterfly spectrum.

2606.06710 2026-06-08 cond-mat.soft 新提交

Beyond Snap-Fit: Optimizing the Lifting Capabilities of a Partial Cylindrical Shell

超越卡扣:优化部分圆柱壳的举升能力

Grace K. Curtis, Ian M. Griffiths, Dominic Vella

AI总结 研究部分圆柱壳作为卡扣的力学行为,通过点力推拉分析接触状态,提出“抓握配合”概念,揭示几何与摩擦对举升性能的影响,为安全举升和易拆卸提供设计原则。

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AI中文摘要

圆柱卡扣是一种普遍存在的紧固方法,既易于制造和装配,又安全可靠。它由一个部分圆柱壳组成,该壳“卡入”圆柱形物体。我们在先前工作的基础上,将圆柱卡扣的力学描述为放置在刚性圆柱体上的自然弯曲薄弹性壳;我们研究了壳在受到点力推拉时的行为。我们根据壳是否具有非零举升能力对可能的接触状态进行分类。我们将具有举升能力的情况称为“抓握配合”,并表明这包括卡扣和“粘附配合”状态,后者虽没有特征性的“卡扣”但允许举升。为完整性起见,还描述了无举升能力的状态。我们表明,不同状态完全由壳/圆柱几何形状和摩擦系数决定。然后,我们考虑了抓握配合状态下举升性能的不同指标。我们的分析揭示了装配力、拆卸力、举升力和夹紧力之间的权衡,为安全举升、易拆卸和易碎物体的安全处理提供了设计原则。

英文摘要

The cylindrical snap-fit is a ubiquitous fastening method that is both simple to manufacture and assemble, and yet secure. It consists of a partial cylindrical shell that `snaps' onto a cylindrical object. We build on previous work to describe the mechanics of the cylindrical snap-fit as a naturally curved thin elastic shell placed atop a rigid cylinder; we investigate the shell's behaviour when subject to a point force pushing it onto or pulling it off the cylinder. We classify the possible contact regimes according to whether the shell has a nonzero lifting capacity. We term situations with lifting capacity `grip-fits' and show that this includes both the snap-fit and a `stick-fit' regime, which allows lifting despite not having the characteristic `snap'. Regimes without lifting capacity are also characterized for completeness. We show that the different regimes may be characterized entirely by the shell/cylinder geometry and the coefficient of friction. We then consider different metrics for the lifting performance in the grip-fit regime. Our analysis reveals the trade-offs between assembly force, disassembly force, lifting force, and clamping force, providing design principles for secure lifting, easy detachment, and safe handling of fragile objects.

2606.06680 2026-06-08 cond-mat.mtrl-sci 新提交

Symmetry-Protected Phonon Topology and Low Lattice Thermal Conductivity in Square-Octagonal Chalcogenides

方八边形硫族化合物中的对称保护声子拓扑和低晶格热导率

Nair Surabhi Suresh, Mondal Chiranjith, Alam Aftab, Singh Nirpendra

AI总结 通过第一性原理和声子玻尔兹曼输运理论,发现方八边形MoS2和SnS单层中对称保护的节点线声子拓扑导致声子软化、群速度抑制和强非谐散射,使晶格热导率相比六方相大幅降低。

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AI中文摘要

非常规晶格几何为实现对称保护拓扑声子态提供了有效平台,这些声子态能强烈影响晶格热输运。在本工作中,我们结合第一性原理计算与声子玻尔兹曼输运理论,探索了方八边形硫族化合物单层(即MoS2和SnS)中拓扑声子带特征与热输运之间的关系。对称性分析揭示了以对称保护节点线形式存在的非平庸声子带拓扑。携带不同对称性本征值的节点线之间的交叉产生了四重狄拉克点,增强了声子群速度(vg),而近乎平坦的节点线则导致vg的强烈抑制。这些特征的共存,加上拓扑带交叉附近显著的声子软化和增强的非谐散射,显著抑制了晶格热导率(κ_l)。因此,室温下so-SnS的κ_l值为4.0 W/mK,so-MoS2为18.7 W/mK,相比其六方相分别降低了超过两倍和八倍。我们的结果揭示了二维材料中声子带拓扑与热输运之间的直接联系,突出了晶格对称性和拓扑带工程作为调控热性能的有前途途径。这些发现进一步为设计具有可控热流的拓扑声子和热电器件提供了机会。

英文摘要

Unconventional lattice geometries provide an effective platform for realizing symmetry-protected topological phonon states that can strongly influence lattice heat transport. In this work, we explore the relationship between topological phonon band features and thermal transport in square--octagonal (so) chalcogenide monolayers, namely MoS2 and SnS, by combining first-principles calculations with phonon Boltzmann transport theory. Symmetry analysis reveals the presence of nontrivial phonon band topology in the form of symmetry-protected nodal lines. Crossings between nodal lines carrying different symmetry eigenvalues produce fourfold Dirac points that enhance the phonon group velocity (vg), whereas nearly flat nodal lines lead to strong suppression of vg. The coexistence of these features, together with substantial phonon softening and enhanced anharmonic scattering around the topological band crossings, markedly suppresses the lattice thermal conductivity ($κ_l$). As a result, room-temperature $κ_l$ values of 4.0 W/mK for so-SnS and 18.7 W/mK for so-MoS2 are obtained, representing reductions by more than a factor of two and eight, respectively, relative to their hexagonal phases. Our results uncover a direct connection between phonon band topology and heat transport in two-dimensional materials, highlighting lattice symmetry and topological band engineering as promising routes for tailoring thermal properties. These findings further suggest opportunities for designing topological phononic and thermoelectric devices with controllable heat flow.

2606.06678 2026-06-08 cond-mat.str-el 新提交

Field-rigid Ising antiferromagnetism with giant spin-flip fields in Van der Waals UOTe

范德瓦尔斯UOTe中的场刚性伊辛反铁磁性与巨自旋翻转场

Zackary Rehfuss, Shannon Gould, Joanna Blawat, Christopher Broyles, George Xu, Yiqing Hao, Huibo Cao, Thao Dinh, Suyang Xu, Dave Graf, John Singleton, Sheng Ran

AI总结 本研究通过磁化率、中子衍射和脉冲场磁化测量,发现范德瓦尔斯材料UOTe在约150K下具有二维伊辛型反铁磁序,并在高达73T的磁场中表现出场刚性行为,实现了高温伊辛序与导电、关联及拓扑电子结构的共存。

Comments 11 pages, 5 figures; Supplemental Material: 6 pages, 17 figures

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AI中文摘要

范德瓦尔斯反铁磁体提供了一条通过厚度控制磁有序的途径,但很少有材料能将高温伊辛序与导电、关联及拓扑电子结构结合起来。这里我们展示UOTe实现了这种结合。磁化率揭示了强各向异性的顺磁响应,而中子衍射确定了在$T_N \simeq 150$ K以下存在c轴反铁磁序,其序参量指数$\beta = 0.14$,接近二维伊辛值。扭矩磁强计进一步表明,在高场转变以下,有序态仍可用单轴反铁磁体很好地描述。高达73 T的脉冲场磁化表明,沿c轴施加非常大的场时,有序态仍能存在,随后进入一个从约50 T开始的宽泛的变磁区域,并在最高测量场下仍未饱和。角度依赖的近程探测器振荡测量表明,变磁不稳定性由沿有序矩方向的场分量决定,为伊辛型场刚性提供了直接证据。因此,UOTe在一种补偿的范德瓦尔斯金属中建立了具有巨自旋翻转场的场刚性伊辛反铁磁体,其中高温c轴序、准二维磁临界性、近藤关联的铀5f杂化、金属输运和对称性允许的拓扑共存于单一材料中。

英文摘要

Van der Waals antiferromagnets provide a route to thickness-controlled magnetic order, but few combine high-temperature Ising order with conducting, correlated, and topological electronic structure. Here we show that UOTe realizes this combination. Magnetic susceptibility reveals a strongly anisotropic paramagnetic response, while neutron diffraction establishes c-axis antiferromagnetic order below $T_N \simeq 150$ K with an order-parameter exponent $β= 0.14$, close to the two-dimensional Ising value. Torque magnetometry further shows that the ordered state remains well described by a uniaxial antiferromagnet below the high-field transition. Pulsed-field magnetization up to 73 T shows that the ordered state survives to very large fields applied along the c axis before entering a broad metamagnetic regime that begins near 50 T, and remains unsaturated at the highest measured field. Angle-dependent proximity detector oscillator measurements show that the metamagnetic instability is set by the field component along the ordered moment direction, providing direct evidence for Ising-like field rigidity. UOTe therefore establishes a field-rigid Ising antiferromagnet with giant spin-flip fields in a compensated Van der Waals metal, where high-temperature c-axis order, quasi-two-dimensional magnetic criticality, Kondo-associated uranium 5f hybridization, metallic transport, and symmetry-enabled topology coexist in a single material.

2606.06659 2026-06-08 cond-mat.quant-gas cond-mat.stat-mech cond-mat.str-el 新提交

Riemann Rarefaction Waves in a Strongly Interacting Fermi Gas

强相互作用费米气体中的黎曼稀疏波

Eric A. Wolf, Martin Zwierlein

AI总结 研究强相互作用费米气体在激波管几何中释放到真空的膨胀,发现幺正区稀疏波动力学自相似且符合欧拉方程,而偏离幺正区时偏差随黏度增加,但自相似性仍近似保持。

Comments 4+3 Pages, 4+3 Figures

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AI中文摘要

我们研究了均匀、强相互作用的费米气体在“激波管”几何中释放到真空的膨胀。在幺正区,气体是尺度不变且几乎无黏的,我们发现产生的稀疏波动力学是自相似的,并且与所有探测温度下的欧拉方程的黎曼解高度一致。在BEC-BCS交叉中探测远离幺正区的相互作用,我们观察到随着黏度增加,与黎曼解的偏差增大。然而,即使在声扩散率增加二十倍的BCS侧,自相似性仍然近似保持。这可能反映了1D纳维-斯托克斯稀疏流在长时间下如何趋近欧拉自相似解。我们的工作证明了强相互作用费米气体在高度可控环境中研究非线性流体动力学的实用性。

英文摘要

We investigate the expansion of a homogeneous, strongly interacting Fermi gas released into vacuum in a ``shock tube'' geometry. At unitarity, where the gas is scale invariant and nearly inviscid, we find that the resulting rarefaction wave dynamics are self-similar and in excellent agreement with Riemann's solution of the Euler equation for all temperatures probed. Probing interactions away from unitarity within the BEC-BCS crossover, we observe increasing deviations from the Riemann solution as viscosity increases. However, even on the BCS side, where the sound diffusivity is increased twenty-fold, self-similarity is still approximately preserved. This may reflect how 1D Navier-Stokes rarefaction flows approach Euler self-similar solutions at long times. Our work demonstrates the utility of strongly interacting Fermi gases for the study of nonlinear hydrodynamics in a highly controllable setting.

2606.06649 2026-06-08 cond-mat.supr-con cond-mat.other cond-mat.quant-gas cond-mat.str-el 新提交

Charge density waves and enhanced superconductivity in the electron-hole gas: a plausible, simple, physically intuitive model

电子-空穴气体中的电荷密度波与增强超导电性:一个合理、简单、物理直观的模型

Carl A Kukkonen

AI总结 本文提出一个简单的两参数模型,研究电子-空穴气体中的电荷密度波和超导电性,发现当质量比M/m≥4.97时,电荷密度波、电子-空穴散射导致的电阻率以及类似BCS的吸引相互作用同时增强,粗略估计超导转变温度可达约275 K。

Comments 22 pages, 10 figures

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AI中文摘要

利用一个简单的、物理动机明确的两参数模型(密度r_s和质量比M/m),研究了由等量电子和带正电费米子(空穴)组成的中性简并等离子体——电子-空穴气体。我们做了两个简化假设但未证明:电子-空穴关联能近似与密度无关,不影响压力或体积模量;电子-空穴对局域场因子的贡献为零,从而允许使用已知的电子气局域场因子。在这些假设下,所有质量比和密度下的相图、不稳定性和有效相互作用都可以通过简单公式计算,并可在笔记本电脑上重现。关键的物理新内容是移动空穴提供的额外屏蔽。单个函数Delta出现在所有有效相互作用和响应函数的分母中。在q=0(压缩率不稳定性)和有限q处Delta的零点附近,三种现象同时增强:电荷密度波(当M/m≥4.97时)、来自电子-空穴散射的大T^2电阻率,以及纯粹电子类比于BCS电子-声子耦合的吸引性电子-电子相互作用。粗略估计的超导转变温度接近室温,在M/m=9时达到约275 K。我们不声称该模型适用于任何特定材料。目的是激发对假设的审视、对未知局域场因子的计算,以及探究这个最小双载流子框架是否映射到真实系统。

英文摘要

A neutral degenerate plasma of equal numbers of electrons and positively charged fermions (holes) -- the electron-hole gas -- is studied using a simple, physically motivated two-parameter model (density r_s and mass ratio M/m). Two simplifying assumptions are made but not proven: the electron-hole correlation energy is approximately independent of density and does not affect the pressure or bulk modulus, and the electron-hole contribution to the local field factors is zero, allowing use of the known electron-gas local field factors. With these assumptions the phase diagram, instabilities, and effective interactions can be calculated for all mass ratios and densities using simple formulae, reproducible on a laptop. The key new physics is the additional screening provided by the mobile holes. A single function Delta appears in the denominator of all effective interactions and response functions. Near the zeros of Delta at q = 0 (compressibility instability) and at finite q, three phenomena are simultaneously enhanced: charge density waves (for M/m >= 4.97), a large T^2 electrical resistivity from electron-hole scattering, and an attractive electron-electron interaction that is the purely electronic analog of BCS electron-phonon coupling. Crudely estimated superconducting transition temperatures approach room temperature, reaching approximately 275 K at M/m = 9. No claim is made that this model applies to any specific material. The aim is to provoke scrutiny of the assumptions, calculation of the unknown local field factors, and investigation of whether this minimal two-carrier framework maps onto real systems.

2606.06623 2026-06-08 cond-mat.mtrl-sci cond-mat.mes-hall physics.app-ph 新提交

Matching Terahertz and Hall Mobilities as a Hallmark of Intrinsic Charge Transport in Metal-Halide Perovskites

匹配太赫兹和霍尔迁移率作为金属卤化物钙钛矿中本征电荷传输的标志

Dmitry R. Maslennikov, Ben P. Carwithen, Vladimir V. Bruevich, Yichao Cai, Davide Nodari, Navendu Mondal, Xijia Zheng, Beier Hu, Nicola Gasparini, Jarvist M. Frost, Vitaly Podzorov, Artem A. Bakulin

AI总结 通过外延CsPbBr3单晶中OPTP与霍尔迁移率的一致性,证明软晶格钙钛矿中本征电荷传输可在毫米尺度实现,并建立本征迁移率基准方法。

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AI中文摘要

在软晶格材料(包括金属卤化物钙钛矿)中,电荷载流子传输通常被认为在不同长度尺度上高度异质,并受到本征(动态)热电子无序和由晶体缺陷、杂质、晶界及表面态引起的外在(静态)无序的共同影响。因此,通过不同电学和光学测量技术报道的载流子迁移率常常不一致,引发了一个关键问题:真正的本征电荷传输机制(即不受静态无序主导的机制)能否在这些材料的宏观单晶中扩展?在这里,我们在一个典型的金属卤化物钙钛矿体系——外延CsPbBr$_{3}$单晶中展示了这样的机制,其中通过光泵浦-太赫兹探针(OPTP)光谱获得的局部迁移率在广泛的实验条件下与宏观传输迁移率定量一致。利用一个专用的器件平台,能够在同一单晶样品上同时进行霍尔效应和OPTP测量,我们获得了约30 cm$^{2}$V$^{-1}$s$^{-1}$的室温迁移率,这是CsPbBr$_{3}$可靠报道的最高值之一。两种技术都揭示了空穴迁移率的类带隙温度依赖性,具有相似的幂指数,证实了相同的本征传输机制支配着超快/局部和稳态/宏观响应。这些结果表明,在软晶格钙钛矿中,无缺陷电荷传输可以在毫米尺度上实现,并为新兴半导体中本征迁移率的基准测试建立了稳健的方法。

英文摘要

Charge-carrier transport in soft-lattice materials, including metal-halide perovskites, is often perceived to be highly heterogeneous across different length scales, and influenced by both the intrinsic (dynamic) thermal electronic disorder and extrinsic (static) disorder due to crystal defects, impurities, grain boundaries, and surface states. As a consequence, the reported carrier mobilities obtained by different electrical and optical measurement techniques frequently disagree, raising a critical question: can a truly intrinsic charge transport regime (that is, a regime not dominated by static disorder) extend across macroscopic single crystals of these materials? Here, we demonstrate such a regime in an exemplary metal-halide perovskite system, epitaxial CsPbBr$_{3}$ single crystals, where the local mobility obtained via optical pump-terahertz probe (OPTP) spectroscopy quantitatively agrees with the macroscopic transport mobility across a broad range of experimental conditions. Using a dedicated device platform that enables concurrent Hall-effect and OPTP measurements on the same single-crystalline sample, we obtain consistent room-temperature mobilities of ~ 30 cm$^{2}$V$^{-1}$s$^{-1}$, among the highest reliably reported for CsPbBr$_{3}$. Both techniques reveal band-like temperature dependence of the hole mobility with similar power exponents, confirming that the same intrinsic transport mechanism governs the ultrafast/local and steady-state/macroscopic responses. These results show that defect-free charge transport is achievable in soft-lattice perovskites on millimetre length scales and establish a robust methodology for benchmarking intrinsic mobility in emerging semiconductors.

2606.06616 2026-06-08 cond-mat.mtrl-sci 新提交

Temperature-Induced Crossover of Coherent Phonon Mechanisms in Chiral 2D Perovskites

手性二维钙钛矿中相干声子机制的温度诱导交叉

Katherine A Koch, Matthew P Hautzinger, Matthew C Beard, Ajay Ram Srimath Kandada

AI总结 通过相位分辨共振脉冲受激拉曼散射,研究手性二维钙钛矿中激子-晶格耦合的实时结构路径,发现温度诱导从场驱动ISRS到布居驱动DECP的交叉,表明温度可主动调控柔性二维框架的激发态结构坐标。

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AI中文摘要

电子激发与晶格自由度之间的耦合从根本上决定了杂化钙钛矿的光电功能。虽然电子激发态的势能面(PES)通常被认为是静态的(尽管受到热无序的调制),但其随温度的结构演化的确切性质仍然难以捉摸。在这里,我们证明了二维金属卤化物钙钛矿中的激发态结构重构是显式温度演化的,受晶格顺应性控制。我们选择了一个具有异常大的温度依赖性键角方差的手性钙钛矿框架,以最大化结构顺应性。通过相位分辨共振脉冲受激拉曼散射,我们测量了相干声子动力学,并解析了激子-晶格修饰的实时结构路径。我们观察到从场驱动的脉冲受激拉曼散射(ISRS)到布居驱动的相干声子位移激发(DECP)的温度诱导交叉。虽然动量驱动的ISRS路径在低温下占主导,但增加的热能软化晶格并增强坐标驱动的位移路径,使激子能够采样激发态PES中更陡峭、高度非简谐的区域。我们的结果表明,温度可以主动调节柔性二维框架的激发态结构坐标,为在手性光电子学中调节激子-晶格相互作用提供了一种实用策略。

英文摘要

The coupling between electronic excitations and lattice degrees of freedom fundamentally dictates the optoelectronic functionality of hybrid perovskites. While the potential energy surfaces (PESs) of the electronic excited states are typically considered static, albeit modulated by thermal disorder, the exact nature of their structural evolution with temperature remains elusive. Here, we demonstrate that the excited-state structural reconfiguration in two-dimensional metal-halide perovskites is explicitly temperature-evolving, governed by lattice compliance. We select a chiral perovskite framework with an exceptionally large, temperature-dependent bond angle variance to maximize the structural compliance. Through phase-resolved resonant impulsive stimulated Raman scattering, we measure the coherent phonon dynamics and resolve the real-time structural pathways of exciton-lattice dressing. We observe a temperature-induced crossover from field-driven Impulsive Stimulated Raman Scattering (ISRS) to population-driven Displacive Excitation of Coherent Phonons (DECP). While momentum-driven ISRS pathways dominate at low temperatures, increasing thermal energy softens the lattice and enhances coordinate-driven displacive pathways, allowing excitons to sample steeper, highly anharmonic regions of the excited-state PES. Our results show that temperature can actively modulate the excited-state structural coordinates of flexible 2D frameworks, offering a practical strategy to tune exciton-lattice interactions in chiral optoelectronics.

2606.06605 2026-06-08 cond-mat.str-el 新提交

Tensor network study of deconfined quantum criticality in a one-dimensional spin-phonon model

一维自旋-声子模型中退禁闭量子临界点的张量网络研究

Anton Romen, Josef Willsher, David Hofmeier, Johannes Knolle, Michael Knap

AI总结 通过张量网络模拟,研究一维反铁磁J1-J2模型中自旋-声子耦合对退禁闭量子临界点的影响,发现低于临界频率时转变变为强一级相变,并识别出有效理论为双正弦-戈登模型。

Comments 18 pages, 14 figures

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AI中文摘要

退禁闭量子临界点(DQCP)描述了超越朗道范式的有序相之间的连续转变。一个简单的例子是一维反铁磁$J_1-J_2$模型中的奈尔反铁磁(AFM)到价键固体(VBS)转变。类似于临界自旋链的自旋-派尔斯不稳定性,DQCP预计在低于临界声子频率时对晶格畸变不稳定。在这项工作中,我们使用张量网络模拟来研究耦合到晶格振动的反铁磁$J_1-J_2$模型中的这种不稳定性。我们确认了DQCP在大声子频率下的稳定性,并证明转变在低于临界频率时变为强一级相变。这种不稳定性是由自旋-声子相互作用导致的Luttinger参数减小引起的,我们将该行为的有效理论识别为双正弦-戈登模型。已知相同的有效理论描述经典Ashkin-Teller模型,这使我们能够证明临界端点属于四态Potts普适类。此外,我们提供了声子谱函数的定量数值标度结果,为在低维材料中探测DQCP-声子耦合提供了实验特征。

英文摘要

Deconfined quantum critical points (DQCPs) describe continuous transitions between ordered phases beyond the Landau paradigm. A simple example is the Néel antiferromagnet (AFM) to valence bond solid (VBS) transition in a 1D antiferromagnetic $J_1-J_2$ model. In analogy to the spin-Peierls instability of critical spin chains, DQCPs are predicted to be unstable towards lattice distortions below a critical phonon frequency. In this work, we use tensor network simulations to investigate this instability in the antiferromagnetic $J_1-J_2$ model coupled to lattice vibrations. We confirm the stability of DQCP for large phonon frequencies and demonstrate that the transition turns strongly first-order below a critical frequency. The instability is caused by a reduction of the Luttinger parameter due to spin-phonon interactions and we identify the effective theory of the behavior as the double sine-Gordon model. The same effective theory is known to describe the classical Ashkin-Teller model, which enables us to show that the critical endpoint is in the four-state Potts universality class. Furthermore, we provide quantitative numerical scaling results for the phonon spectral function, offering an experimental signature to probe DQCP-phonon coupling in low-dimensional materials.

2606.06584 2026-06-08 cond-mat.str-el 新提交

Bootstrap bounds for Quantum Spin Systems using String Operators

使用弦算子的量子自旋系统的自举界

Nisarg Chadha, Michael G. Scheer, Eslam Khalaf

AI总结 引入非局域弦算子到自举法中,在热力学极限下直接公式化,显著收紧1D横场Ising模型SSB相的界,并用于定量估计相边界位置。

Comments 9 pages, 4 figures

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AI中文摘要

自举是一种数值多体方法,通过施加对算符期望值的一组必要约束,为基态可观测量提供严格的界。所得界的质量对进入约束的算符选择敏感。特别是,在自发对称性破缺(SSB)相中,基态关联的界通常较松,因为局域算符集无法排除畴壁激发。在这项工作中,我们将非局域的弦状算符引入自举,并展示该程序可以直接在热力学极限下公式化。然后,我们将我们的构造应用于几个一维自旋模型。首先,我们在1D横场Ising模型的SSB相中获得了界的显著收紧。利用1D轴向次近邻Ising模型,我们进一步展示了这种收紧允许对相边界位置进行定量估计。最后,我们将弦算子推广到1D $\mathbb{Z}_3$ 手征时钟模型,并追踪界在整个相图中的行为。我们的结果拓宽了自举可用的约束类别,并为自举更一般的对称破缺和拓扑相开辟了道路,其中相关约束可能涉及非局域或扩展算子。

英文摘要

Bootstrap is a numerical many-body method that provides rigorous bounds on ground-state observables by imposing a set of necessary constraints on the expectation values of operators. The quality of the resulting bounds is sensitive to the choice of operators entering the constraints. In particular, bounds on ground-state correlations are often loose in spontaneous symmetry-breaking (SSB) phases, since local operator sets cannot exclude domain-wall excitations. In this work, we introduce non-local, string-like operators into the bootstrap and show that the program can be formulated directly in thermodynamic limit. We then apply our construction to several 1D spin models. First, we obtain a significant tightening of the bounds in the SSB phase of the 1D transverse-field Ising model. Using the 1D axial next-nearest-neighbor Ising model, we further show that this tightening allows for a quantitative estimate of the locations of phase boundaries. Finally, we generalize the string operators to the 1D $\mathbb{Z}_3$ chiral clock model and track the behavior of the bounds across the phase diagram. Our results broaden the class of constraints available to the bootstrap and open a route toward bootstrapping more general symmetry-broken and topological phases, where the relevant constraints may involve non-local or extended operators.