Coherent room-temperature dipole synchronization in nanocavity sheets
纳米腔薄片中的室温偶极子同步
Rakesh Arul, Piper Fowler-Wright, Lille Borresen, Brendon W. Lovett, Jonathan Keeling, Jeremy J. Baumberg
AI总结 本文报道在非共振连续波泵浦下,局域有序等离子体纳米间隙二维阵列中形成室温同步偶极子态,该体系通过近场强耦合实现空间偶极子同步,但快速辐射和非辐射发射抑制时间光子相干性,为室温同步研究提供新平台。
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等离子体纳米腔能够通过亚纳米间隙中的强近场耦合实现空间分离的发射偶极子的同步。我们报道了在非共振连续波泵浦下,局域有序等离子体纳米间隙二维阵列中形成室温同步偶极子态。与激光、光子玻色-爱因斯坦凝聚或激子-极化激元凝聚不同,该体系在偶极子间展现出空间相干性,而快速的辐射和非辐射发射抑制了时间光子相干性。随着泵浦增加,观察到行为变化,表现为g(1)相干性的空间扩展,但没有光谱窄化或定向发射。这种驱动-耗散体系展现出快速的时间相干衰减和复杂的空间关联,为研究室温同步提供了新平台。结合超低模式体积、高Purcell增强和可扩展的环境操作,它为新型光子和量子技术开辟了道路。
Plasmonic nanocavities enable the synchronization of spatially distant emissive dipoles through strong near-field coupling in sub-nm gaps. We report formation of a room-temperature synchronized dipole state in locally-ordered plasmonic nanogap 2D arrays under non-resonant continuous-wave pumping. Unlike lasers, photonic Bose-Einstein condensates, or exciton-polariton condensates, this system exhibits spatial coherence across the dipoles, while rapid radiative and non-radiative emission suppresses temporal photon coherence. A change of behaviour is observed with increasing pumping, marked by the spatial spread of g(1) coherence, but without spectral narrowing or directional emission. This driven-dissipative system exhibits fast temporal coherence decay and complex spatial correlations, offering a new platform for studying synchronization at room temperature. Combining ultralow mode volumes, high Purcell enhancement, and scalable ambient operation, it opens pathways for novel photonic and quantum technologies.